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Evolution of charge order in the hole-doped kagome superconductor CsV<sub>3</sub>Sb<sub>5</sub>

ORAL

Abstract

We present a study of charge density wave (CDW) orders with hole doping in the kagome lattice sites of CsV3Sb5, utilizing high dynamic range single crystal X-ray diffraction (SCXRD) measurements. Vanadium atoms are replaced with controlled amounts of Titanium atoms using a conventional flux-based single-crystal growth technique to achieve hole doping in the kagome sites. We examine the progression of charge correlations upon the suppression of long-range charge density wave order as the doping level transitions from the first superconducting dome to the second superconducting dome in CsV3-xTixSb5. Our data indicates that the 2×2×2 supercell is more robust than the 2×2×4 supercell, remaining stable at relatively higher Ti-doping levels. At a doping level of x = 0.15, within the region of the second superconducting dome, no superlattice peaks are detected, revealing a complete suppression of charge correlations. Our work reveals the intricate interplay between unconventional superconductivity and the charge density waves correlations with hole doping in the kagome sites of CsV3Sb5

Presenters

  • Ganesh Pokharel

    University of West Georgia, University of California, Santa Barbara

Authors

  • Ganesh Pokharel

    University of West Georgia, University of California, Santa Barbara

  • Brenden R Ortiz

    Oak Ridge National Laboratory

  • Andrea C Salinas

    University of California, Santa Barbara, University of California Santa Barbara, University of Maryland College Park

  • Steven J Gomez Alvarado

    University of California, Santa Barbara, Materials Department, University of California, Santa Barbara, CA 93106-5050, U.S.A.

  • Jacob Ruff

    Cornell High Energy Synchrotron Source

  • Suchismita Sarker

    Cornell High Energy Synchrotron Source, CHESS, Cornell University, Cornell

  • Stephen D Wilson

    University of California, Santa Barbara