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Near-room-temperature ferromagnetic ordering in the pressure-induced collapsed-tetragonal phase in SrCo<sub>2</sub>P<sub>2</sub>

ORAL

Abstract

We present high-pressure electrical transport, magnetization, and single-crystal X-ray diffraction data on SrCo2P2. X-ray diffraction shows a transition to a collapsed tetragonal (cT) structure above ~10 GPa, with the resistance measurement revealing a clear transition-like feature up to 260 K. Magnetization, magnetoresistance, and Hall measurements indicate the transition leads to a ferromagnetic ground state. Density functional theory (DFT) calculations support a first-order transition between tetragonal and cT phases at ~10 GPa and show the emergence of ferromagnetic ordering in the cT phase. Above ~30 GPa, magnetic ordering vanishes in a first-order-like manner, consistent with theoretical predictions, suggesting SrCo2P2 is another sample of ferromagnetic intermetallic compound that avoids quantum criticality.

Presenters

  • Raquel A. Ribeiro

    Iowa State University

Authors

  • Raquel A. Ribeiro

    Iowa State University

  • Shuyuan huyan

    Ames National Laboratory

  • Juan Schmidt

    Ames National Laboratory, Ames National Laboratory, and Department of Physics and Astronomy, Iowa State University

  • Juan Schmidt

    Ames National Laboratory, Ames National Laboratory, and Department of Physics and Astronomy, Iowa State University

  • Adrian Valadkhani

    Goethe University Frankfurt

  • Haozhe Wang

    Michigan State University

  • Zhuoqi Li

    Ames National Laboratory

  • Aashish Sapkota

    Ames National Laboratory

  • James L Petri

    University of Alabama at Birmingham

  • Tyler J Slade

    Ames National Laboratory

  • Wenli Bi

    University of Alabama at Birmingham

  • Weiwei Xie

    Michigan State University

  • Igor I Mazin

    George Mason University, George Mason University, Quantum Science and Engineering Center, Depertment of Physics and Astronomy, George Mason University; Quantum Science and Engineering Centre, George Mason University

  • Roser Valenti

    Goethe University Frankfurt, Frankfurt

  • Sergey L Bud'ko

    Iowa State University, Ames National Laboratory, and Department of Physics and Astronomy, Iowa State University, Ames National Laboratory and Iowa State University

  • Paul C Canfield

    Iowa State University, Ames National Laboratory, and Department of Physics and Astronomy, Iowa State University, Ames National Laboratory and Iowa State University