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Resilient spin dynamics in Y-doped TbSb near percolation limits

ORAL

Abstract

Understanding disorder in magnetic systems and designing materials with disorder resistant spinwaves is crucial for spintronics and magnonics. An effective model system for exploring magnetic disorder through non-magnetic element doping is hosted by cubic crystal structures like TbSb (S = 7/2, 9.7 μB). Y-doping in TbSb lowers the Néel temperature and allows for investigating the interplay between disorder and magnetic excitations across different doping concentrations. We examine the impact of Y-doping on magnetic excitations in TbSb using inelastic neutron scattering and SU(N) generalized spinwave modelling. With increasing Y concentration, magnons in TbSb gradually soften even upto its percolation threshold of 40% Y-doping. Surprisingly, magnons at 40% Y-doping survives even above the Néel temperature, even though it is expected to undergo paramagnon transition as in the case of pure TbSb. Simulations based on SU(N) generalized spinwave theory reveal how spin waves and crystal field excitations evolve with doping. Our study offers new insights into magnon behavior in disordered magnetic systems, emphasizing opportunities for deeper exploration in this field.

Presenters

  • George Yumnam

    Oak Ridge National Laboratory

Authors

  • George Yumnam

    Oak Ridge National Laboratory

  • David Adam Dahlbom

    Oak Ridge National Laboratory, University of Tennessee

  • Duncan H. Moseley

    Oak Ridge National Laboratory

  • H. Suriya W Arachchige

    University of Tennessee, Knoxville, Unknown

  • Barry Winn

    Oak Ridge National Laboratory

  • Allen O Scheie

    Los Alamos National Laboratory (LANL)

  • David G Mandrus

    University of Tennessee

  • Wei Tian

    Oak Ridge National Laboratory, ORNL

  • Michael E Manley

    Oak Ridge National Laboratory

  • Daniel M Pajerowski

    Oak Ridge National Laboratory

  • Raphael Pierre Hermann

    Oak Ridge National Laboratory