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Effect of interlayer coupling in charge transport across strongly disordered multilayer reduced graphene oxide

ORAL

Abstract

Charge transport across disordered multilayers, especially the precise role of interlayer interaction in promoting or jeopardizing electron flow, remains unclear. This work investigates charge transport across multilayer graphene oxide using a multiscale computational approach, which bridges first-principles calculations with large-scale transport simulations. It is observed that resistivity deviates from the well-known scaling laws. Also, the hierarchy of transport regimes between diffusion and localization is reversed. A scaling law for resistivity depending on the number of layers is proposed. The predictions compare very well with the experimental data and are valid not only for reduced graphene oxide but for other multilayer 2D materials, as well. [1]

Publication: M. N. Cinar, A. Antidormi, V.-H. Nguyen, A. Kovtun, S. Lara-Avila, A. Liscio, J.-C. Charlier, S. Roche, H. Sevinçli, "Toward Optimized Charge Transport in Multilayer Reduced Graphene Oxides" Nano Lett. 22, 2202 (2022)

Presenters

  • Haldun Sevincli

    Bilkent University

Authors

  • Haldun Sevincli

    Bilkent University

  • Mustafa Neset Cinar

    Izmir Institute of Technology

  • Aleandro Antidormi

    Catalan Institute of Nanoscience and Nanotechnology, CSIC and The Barcelona Institute of Science and Technology, Campus UAB, 08193 Bellaterra, Barcelona, Spain

  • Viet-Hung Nguyen

    Institute of Condensed Matter and Nanosciences, Université catholique de Louvain (UCLouvain), B-1348 Louvain-la-Neuve, Belgium

  • Alessandro Kovtun

    Consiglio Nazionale delle Ricerche, Istituto per la Sintesi Organica e la Fotoreattivitá, (CNR-ISOF), via Gobetti 101, 40129 Bologna, Italy

  • Samuel Lara-Avila

    Department of Microtechnology and Nanoscience, Chalmers University of Technology, Kemivägen 9, 41296 Gothenburg, Sweden

  • Andrea Liscio

    Consiglio Nazionale delle Ricerche, Istituto per la Microelettronica e Microsistemi, Roma Unit (CNR-IMM), via del fosso del cavaliere 100, 00133 Rome, Italy

  • Jean-Christophe Charlier

    Institute of Condensed Matter and Nanosciences, Université catholique de Louvain (UCLouvain), B-1348 Louvain-la-Neuve, Belgium

  • Stephan Roche

    Catalan Institute of Nanoscience and Nanotechnology, CSIC and The Barcelona Institute of Science and Technology, Campus UAB, 08193 Bellaterra, Barcelona, Spain