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Spin Excitation Continuum in the Exactly Solvable Triangular-Lattice Spin Liquid CeMgAl<sub>11</sub>O<sub>19</sub>

ORAL

Abstract

In magnetically ordered insulators, elementary quasiparticles manifest as spin waves - collective motions of localized magnetic moments propagating through the lattice - observed via inelastic neutron scattering. In effective spin-1/2 systems where geometric frustrations suppress static magnetic order, spin excitation continua can emerge, either from degenerate classical spin ground states or from entangled quantum spins characterized by emergent gauge fields and deconfined fractionalized excitations. Comparing the spin Hamiltonian with theoretical models can unveil the microscopic origins of these zero-field spin excitation continua. Here, we use neutron scattering to study spin excitations of the two-dimensional (2D) triangular-lattice effective spin-1/2 antiferromagnet CeMgAl11O19. Analyzing the spin waves in the field-polarized ferromagnetic state, we find that the spin Hamiltonian is close to an exactly solvable 2D triangular-lattice XXZ model, where degenerate 120 ordered ground states - umbrella states - develop in the zero temperature limit. We then find that the observed zero-field spin excitation continuum matches the calculated ensemble of spin waves from the umbrella state manifold, and thus conclude that CeMgAl11O19 is the first example of an exactly solvable spin liquid on a triangular lattice where the spin excitation continuum arises from the ground state degeneracy.

Publication: arXiv:2408.15957

Presenters

  • Bin Gao

    Rice University

Authors

  • Bin Gao

    Rice University

  • Tong Chen

    Johns Hopkins University

  • Chunxiao Liu

    University of California, Berkeley

  • Mason L Klemm

    Rice University

  • Shu Zhang

    Max Planck Institute for the Physics of Complex Systems

  • Zhen Ma

    Hubei Normal University

  • Xianghan Xu

    University of Minnesota, Twin Cities, Princeton University

  • Choongjae Won

    Pohang Univ of Sci & Tech

  • Gregory T McCandless

    Baylor University

  • Naoki Murai

    Japan Atomic Energy Agency

  • Seiko Ohira-Kawamura

    Japan Atomic Energy Agency

  • Stephen John Moxim

    National Institute of Standards and Technology (NIST)

  • Jason Ryan

    National Institute of Standards and Technology (NIST)

  • Xiaozhou Huang

    Argonne National Laboratory

  • Xiaoping Wang

    Oak Ridge National Laboratory

  • Julia Y Chan

    Baylor Univeristy, Baylor University, Balor University

  • Sang-Wook Cheong

    Rutgers University

  • Oleg V Tchernyshyov

    Johns Hopkins University

  • Leon Balents

    University of California, Santa Barbara

  • Pengcheng Dai

    Rice University