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Er-implanted WS2 flakes with room-temperature photon emission at telecom wavelengths

ORAL

Abstract

Rare earth ions in solids promise applications in quantum communication and nanoscale sensing, but circumventing constraints imposed by the material host often prove challenging. In this work we combine ion implantation, IR confocal microscopy, and ab-initio calculations to demonstrate room-temperature telecom emission of Er3+ in exfoliated WS2 flakes. Confocal microscopy and optical spectroscopy reveal narrow, long-lived photoluminescence that activates after low-temperature thermal annealing. Polarization-selective measurements show a uniform response across the flakes, suggesting Er ions take equivalent positions in the WS2 lattice, possibly substituting tungsten. Quantum embedding calculations of ErW yield a set of PL lines in the telecom band, qualitatively consistent with our experimental observations. Our results create opportunities for novel solid-state devices coupling 2D-hosted, telecom-band emitters.

Publication: Er-implanted WS 2 flakes with room-temperature photon emission at telecom wavelengths, Guadalupe García Arellano, Gabriel I. López Morales, Zav Shotan, Raman Kumar, Benedict Murdin, Cyrus Dreyer, and Carlos A. Meriles, article in preparation (we plan to submit to Nanoletters).

Presenters

  • Guadalupe Garcia Arellano

    City College of New York

Authors

  • Guadalupe Garcia Arellano

    City College of New York

  • Gabriel I Lopez Morales

    Stony Brook University, City College of New York

  • Zav Shotan

    City College of New York

  • Raman Kumar

    City College of New York

  • Benedict N Murdin

    University of Surrey

  • Cyrus E Dreyer

    Stony Brook University (SUNY)

  • Carlos Andres Meriles

    City College of New York