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Backfolded acoustic phonons as ultrasonic probes in metal-oxide superlattices

ORAL

Abstract

Ultrasound has been widely used as an incisive probe of internal interfaces. For thin-film structures however, it is largely ineffective because the signal is dominated by the substrate. Using confocal Raman spectro-microscopy, we show that multiple reflection of sound waves at internal interfaces of a metal-oxide superlattice generates standing waves that are insensitive to the substrate. These backfolded acoustic phonon modes are sensitive to atomic-scale thickness variations of the sublayers and thus serve as a powerful characterization tool for metal-oxide superlattices.

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Authors

  • Fryderyk Lyzwa

    Department of Physics and Fribourg Center for Nanomaterials, University of Fribourg, Chemin du Musée 3, CH-1700 Fribourg, Switzerland

  • Anuradha Gupta

    New Jersey Inst of Tech, Pennsylvania State University, Bard College, University of Mississippi, Drexel Univ, Collaborator, University of Dayton, Morgan State University, Louisiana State University, University of Geneva, Instituto Superior Tecnico - Lisboa, Department of Biochemistry and Molecular Biology, Rutgers University, Institute for Quantitative Biomedicine, Rutgers University, Pennsylvania State University, and University of Illinois at Urbana-Champaign, University of Illinois at Urbana-Champaign, Department of Chemical Engineering, New Jersey Institute of Technology, Department of Physics and Astronomy, Rutgers University-New Brunswick, Department of Physics, Rutgers University, Max-Planck-Institut für Festkörperforschung, Heisenbergstrasse 1, 70569 Stuttgart, Germany, Department of Physics and Fribourg Center for Nanomaterials, University of Fribourg, Chemin du Musée 3, CH-1700 Fribourg, Switzerland, The MacDiarmid Institute for Advanced Materials and Nanotechnology, 1010 Auckland, New Zealand, Department of Physics, College of William & Mary, Williamsburg, VA 23187-8795, USA, New Jersey Institute of Technology, Newark, NJ, USA, University of California, Los Angeles, CA, USA, University of California, Berkeley, CA, USA, Space Research Institute of RAS, Moscow, Russia, Georgetown University, Institut Polytechnique de Paris, University of Delaware, Brookhaven National Laboratory, San Diego State University, University of Chicago, University of Illinois at Chicago, Argonne National Laboratory, Department of Physics and Astronomy, Rutgers University, Piscataway, NJ 08854, USA, University of Washington

  • Anuradha Gupta

    New Jersey Inst of Tech, Pennsylvania State University, Bard College, University of Mississippi, Drexel Univ, Collaborator, University of Dayton, Morgan State University, Louisiana State University, University of Geneva, Instituto Superior Tecnico - Lisboa, Department of Biochemistry and Molecular Biology, Rutgers University, Institute for Quantitative Biomedicine, Rutgers University, Pennsylvania State University, and University of Illinois at Urbana-Champaign, University of Illinois at Urbana-Champaign, Department of Chemical Engineering, New Jersey Institute of Technology, Department of Physics and Astronomy, Rutgers University-New Brunswick, Department of Physics, Rutgers University, Max-Planck-Institut für Festkörperforschung, Heisenbergstrasse 1, 70569 Stuttgart, Germany, Department of Physics and Fribourg Center for Nanomaterials, University of Fribourg, Chemin du Musée 3, CH-1700 Fribourg, Switzerland, The MacDiarmid Institute for Advanced Materials and Nanotechnology, 1010 Auckland, New Zealand, Department of Physics, College of William & Mary, Williamsburg, VA 23187-8795, USA, New Jersey Institute of Technology, Newark, NJ, USA, University of California, Los Angeles, CA, USA, University of California, Berkeley, CA, USA, Space Research Institute of RAS, Moscow, Russia, Georgetown University, Institut Polytechnique de Paris, University of Delaware, Brookhaven National Laboratory, San Diego State University, University of Chicago, University of Illinois at Chicago, Argonne National Laboratory, Department of Physics and Astronomy, Rutgers University, Piscataway, NJ 08854, USA, University of Washington

  • Anuradha Gupta

    New Jersey Inst of Tech, Pennsylvania State University, Bard College, University of Mississippi, Drexel Univ, Collaborator, University of Dayton, Morgan State University, Louisiana State University, University of Geneva, Instituto Superior Tecnico - Lisboa, Department of Biochemistry and Molecular Biology, Rutgers University, Institute for Quantitative Biomedicine, Rutgers University, Pennsylvania State University, and University of Illinois at Urbana-Champaign, University of Illinois at Urbana-Champaign, Department of Chemical Engineering, New Jersey Institute of Technology, Department of Physics and Astronomy, Rutgers University-New Brunswick, Department of Physics, Rutgers University, Max-Planck-Institut für Festkörperforschung, Heisenbergstrasse 1, 70569 Stuttgart, Germany, Department of Physics and Fribourg Center for Nanomaterials, University of Fribourg, Chemin du Musée 3, CH-1700 Fribourg, Switzerland, The MacDiarmid Institute for Advanced Materials and Nanotechnology, 1010 Auckland, New Zealand, Department of Physics, College of William & Mary, Williamsburg, VA 23187-8795, USA, New Jersey Institute of Technology, Newark, NJ, USA, University of California, Los Angeles, CA, USA, University of California, Berkeley, CA, USA, Space Research Institute of RAS, Moscow, Russia, Georgetown University, Institut Polytechnique de Paris, University of Delaware, Brookhaven National Laboratory, San Diego State University, University of Chicago, University of Illinois at Chicago, Argonne National Laboratory, Department of Physics and Astronomy, Rutgers University, Piscataway, NJ 08854, USA, University of Washington

  • Anuradha Gupta

    New Jersey Inst of Tech, Pennsylvania State University, Bard College, University of Mississippi, Drexel Univ, Collaborator, University of Dayton, Morgan State University, Louisiana State University, University of Geneva, Instituto Superior Tecnico - Lisboa, Department of Biochemistry and Molecular Biology, Rutgers University, Institute for Quantitative Biomedicine, Rutgers University, Pennsylvania State University, and University of Illinois at Urbana-Champaign, University of Illinois at Urbana-Champaign, Department of Chemical Engineering, New Jersey Institute of Technology, Department of Physics and Astronomy, Rutgers University-New Brunswick, Department of Physics, Rutgers University, Max-Planck-Institut für Festkörperforschung, Heisenbergstrasse 1, 70569 Stuttgart, Germany, Department of Physics and Fribourg Center for Nanomaterials, University of Fribourg, Chemin du Musée 3, CH-1700 Fribourg, Switzerland, The MacDiarmid Institute for Advanced Materials and Nanotechnology, 1010 Auckland, New Zealand, Department of Physics, College of William & Mary, Williamsburg, VA 23187-8795, USA, New Jersey Institute of Technology, Newark, NJ, USA, University of California, Los Angeles, CA, USA, University of California, Berkeley, CA, USA, Space Research Institute of RAS, Moscow, Russia, Georgetown University, Institut Polytechnique de Paris, University of Delaware, Brookhaven National Laboratory, San Diego State University, University of Chicago, University of Illinois at Chicago, Argonne National Laboratory, Department of Physics and Astronomy, Rutgers University, Piscataway, NJ 08854, USA, University of Washington

  • Anuradha Gupta

    New Jersey Inst of Tech, Pennsylvania State University, Bard College, University of Mississippi, Drexel Univ, Collaborator, University of Dayton, Morgan State University, Louisiana State University, University of Geneva, Instituto Superior Tecnico - Lisboa, Department of Biochemistry and Molecular Biology, Rutgers University, Institute for Quantitative Biomedicine, Rutgers University, Pennsylvania State University, and University of Illinois at Urbana-Champaign, University of Illinois at Urbana-Champaign, Department of Chemical Engineering, New Jersey Institute of Technology, Department of Physics and Astronomy, Rutgers University-New Brunswick, Department of Physics, Rutgers University, Max-Planck-Institut für Festkörperforschung, Heisenbergstrasse 1, 70569 Stuttgart, Germany, Department of Physics and Fribourg Center for Nanomaterials, University of Fribourg, Chemin du Musée 3, CH-1700 Fribourg, Switzerland, The MacDiarmid Institute for Advanced Materials and Nanotechnology, 1010 Auckland, New Zealand, Department of Physics, College of William & Mary, Williamsburg, VA 23187-8795, USA, New Jersey Institute of Technology, Newark, NJ, USA, University of California, Los Angeles, CA, USA, University of California, Berkeley, CA, USA, Space Research Institute of RAS, Moscow, Russia, Georgetown University, Institut Polytechnique de Paris, University of Delaware, Brookhaven National Laboratory, San Diego State University, University of Chicago, University of Illinois at Chicago, Argonne National Laboratory, Department of Physics and Astronomy, Rutgers University, Piscataway, NJ 08854, USA, University of Washington

  • Anuradha Gupta

    New Jersey Inst of Tech, Pennsylvania State University, Bard College, University of Mississippi, Drexel Univ, Collaborator, University of Dayton, Morgan State University, Louisiana State University, University of Geneva, Instituto Superior Tecnico - Lisboa, Department of Biochemistry and Molecular Biology, Rutgers University, Institute for Quantitative Biomedicine, Rutgers University, Pennsylvania State University, and University of Illinois at Urbana-Champaign, University of Illinois at Urbana-Champaign, Department of Chemical Engineering, New Jersey Institute of Technology, Department of Physics and Astronomy, Rutgers University-New Brunswick, Department of Physics, Rutgers University, Max-Planck-Institut für Festkörperforschung, Heisenbergstrasse 1, 70569 Stuttgart, Germany, Department of Physics and Fribourg Center for Nanomaterials, University of Fribourg, Chemin du Musée 3, CH-1700 Fribourg, Switzerland, The MacDiarmid Institute for Advanced Materials and Nanotechnology, 1010 Auckland, New Zealand, Department of Physics, College of William & Mary, Williamsburg, VA 23187-8795, USA, New Jersey Institute of Technology, Newark, NJ, USA, University of California, Los Angeles, CA, USA, University of California, Berkeley, CA, USA, Space Research Institute of RAS, Moscow, Russia, Georgetown University, Institut Polytechnique de Paris, University of Delaware, Brookhaven National Laboratory, San Diego State University, University of Chicago, University of Illinois at Chicago, Argonne National Laboratory, Department of Physics and Astronomy, Rutgers University, Piscataway, NJ 08854, USA, University of Washington

  • Benjamin P. P. Mallett

    The MacDiarmid Institute for Advanced Materials and Nanotechnology, 1010 Auckland, New Zealand