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Dark field x-ray microscopy for mesoscale phenomena in ordered quantum, structural, and functional materials at modern light sources

ORAL

Abstract

Single-crystal diffraction reveals an ‘average’ view of ordered materials; in contrast, dark field x-ray microscopy (DFXM) provides real-space images of mesoscale inhomogeneities that encode spatial information on a Bragg, or a super-lattice (e.g. charge-density wave, magnetic order) peak. In DFXM, a lens magnifies a Bragg peak exiting a sample to form an image. DFXM carried out concurrently with in situ multi-modal measurements can shed light on underlying correlations of materials properties to mesoscale features. Some examples are presented to illustrate the potency of DFXM and introduce cryogenic and associated instrumentation.

Publication: Zhi Qiao, Xianbo Shi, Peter Kenesei, Arndt Last, Lahsen Assoufid, and Zahir Islam, "A large field-of-view high-resolution hard x-ray microscope using polymer optics," Rev. Sci. Instrum. 91, 113703 (2020); https://doi.org/10.1063/5.0011961; Ishwor Poudyal, Zhi Qiao, Michael R. Armstrong, and Zahir Islam, "Pump-probe dark-field x-ray microscopy", arXiv:2210.06243v1, cond-mat.mtrl-sci, (2022).

Presenters

  • Zahir Islam

    Argonne National Laboratory

Authors

  • Zahir Islam

    Argonne National Laboratory

  • Elliot S Kisiel

    University of California, San Diego

  • Jayden C Plumb

    UC Santa Barbara; Argonne National Laboratory

  • Omar Shohoud

    Argonne National Laboratory

  • Ishwor Poudyal

    Materials Science Division, Argonne National Laboratory

  • Zhan Zhang

    Argonne National Laboratory, argonne national laboratory

  • Siddarth Maddali

    Argonne National Laboratory

  • Stephan O Hruszkewycz

    Argonne National Laboratory