Z4 Electronic Fractals in NdNiO<sub>3</sub>
ORAL
Abstract
Rare-earth nickelates have a phase diagram characterized by overlapping electronic, structural
and magnetic phase transitions. In the vicinity of critical points, local maps of the associated
order parameter exhibit complex pattern formation. We simulate a clean 2D 4-state clock model
near the phase transition temperature. We also cool 2D random field 4-state clock models using the
Metropolis algorithm and find that they reach a glassy state. From the patterns of magnetic domains
at the phase transition in the 2D clean 4-state clock model and the 2D random field clock model, we
calculate critical exponents for the cluster size distribution, volume fractal dimension, hull fractal
dimension and pair connectivity function. We compare these exponents to the exponents extracted
from antiferromagnetic domains in NdNiO3 using resonant magnetic X-ray scattering nanoprobe
measurements [Li et al., Nat. Commun., 2019]. The four types of magnetic domains in NdNiO3
follow a Z4 symmetry, and we model the symmetry breaking in the ordered phase with 4-state clock
models. The power law scaling of the cluster properties and pair connectivity correlation function
demonstrates that the observed patterns in NdNiO3 are fractals. We find that the critical exponents
from the 2D random field 4-state clock model are consistent with the critical exponents measured
in NdNiO3. This indicates that the paramagnet-antiferromagnet transition in rare earth nickelates
is in the same universality class as the 4-state random field clock model
and magnetic phase transitions. In the vicinity of critical points, local maps of the associated
order parameter exhibit complex pattern formation. We simulate a clean 2D 4-state clock model
near the phase transition temperature. We also cool 2D random field 4-state clock models using the
Metropolis algorithm and find that they reach a glassy state. From the patterns of magnetic domains
at the phase transition in the 2D clean 4-state clock model and the 2D random field clock model, we
calculate critical exponents for the cluster size distribution, volume fractal dimension, hull fractal
dimension and pair connectivity function. We compare these exponents to the exponents extracted
from antiferromagnetic domains in NdNiO3 using resonant magnetic X-ray scattering nanoprobe
measurements [Li et al., Nat. Commun., 2019]. The four types of magnetic domains in NdNiO3
follow a Z4 symmetry, and we model the symmetry breaking in the ordered phase with 4-state clock
models. The power law scaling of the cluster properties and pair connectivity correlation function
demonstrates that the observed patterns in NdNiO3 are fractals. We find that the critical exponents
from the 2D random field 4-state clock model are consistent with the critical exponents measured
in NdNiO3. This indicates that the paramagnet-antiferromagnet transition in rare earth nickelates
is in the same universality class as the 4-state random field clock model
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Presenters
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Forrest Simmons
Purdue University
Authors
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Forrest Simmons
Purdue University
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Jiarui Li
Massachusetts Institute of Technology MIT
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Jonathan Pelliciari
Massachusetts Institute of Technology MIT
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Claudio Mazzoli
Brookhaven National Laboratory
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Sara Catalano
DQMP, University of Geneva
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Jerzy Sadowski
Brookhaven National Laboratory, Brookhaven National Lab
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Abraham L Levitan
Massachusetts Institute of Technology
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Marta Gibert
Univ of Zurich
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Erica W Carlson
Purdue University
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Jean-Marc Triscone
Univ of Geneva
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Stuart Wilkins
Brookhaven National Laboratory
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Riccardo Comin
Massachusetts Institute of Technology MIT, Massachusetts Institute of Technology