Noncoplanar Spin Textures in Cubic Double Perovskites Ba<sub>2</sub>YRuO<sub>6</sub> and Ba<sub>2</sub>LuRuO<sub>6</sub>
ORAL
Abstract
Magnetic materials with noncoplanar magnetic structures can show unusual physical properties driven by nontrivial topology. Topologically-active states are often multi-q structures, which are challenging to stabilize in models and to identify in materials. In this talk, we use inelastic neutron-scattering data to show that the insulating double perovskites Ba2YRuO6 and Ba2LuRuO6-- previously assumed to be collinear antiferromagnets -- actually host a noncoplanar triple-q structure on the face-centered cubic lattice. I discuss the magnetic interactions that may stabilize this state, considering biquadratic exchange and cubic anisotropy. Our work identifies cubic double perovskites as a promising class of materials to realize topological magnetic states, elucidates the likely stabilization mechanism of the triple-q state in these materials, and establishes neutron spectroscopy on powder samples as a valuable technique to distinguish multi-q from single-q structures, facilitating the discovery of topologically-nontrivial magnetic materials.
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Presenters
Joe Paddison
Oak Ridge National Lab, Oak Ridge National Laboratory
Authors
Joe Paddison
Oak Ridge National Lab, Oak Ridge National Laboratory
Jiaqiang Yan
Oak Ridge National Laboratory, Materials Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA
Hao Zhang
University of Tennessee
Seunghwan Do
Oak Ridge National Laboratory
Shang Gao
Oak Ridge National Laboratory, Department of Physics, University of Science and Technology of China
Matthew B Stone
Oak Ridge National Lab, Oak Ridge National Laboratory
David A Dahlbom
University of Tennessee, University of Tennessee, Knoxville
Kipton M Barros
Los Alamos Natl Lab, Theoretical Division and CNLS, Los Alamos National Laboratory
Cristian Batista
University of Tennessee, University of Tennessee, Knoxville
Andy Christianson
Oak Ridge National Laboratory, Oak Ridge National Lab