APS Logo

Noncoplanar Spin Textures in Cubic Double Perovskites Ba<sub>2</sub>YRuO<sub>6</sub> and Ba<sub>2</sub>LuRuO<sub>6</sub>

ORAL

Abstract

Magnetic materials with noncoplanar magnetic structures can show unusual physical properties driven by nontrivial topology. Topologically-active states are often multi-q structures, which are challenging to stabilize in models and to identify in materials. In this talk, we use inelastic neutron-scattering data to show that the insulating double perovskites Ba2YRuO6 and Ba2LuRuO6 -- previously assumed to be collinear antiferromagnets -- actually host a noncoplanar triple-q structure on the face-centered cubic lattice. I discuss the magnetic interactions that may stabilize this state, considering biquadratic exchange and cubic anisotropy. Our work identifies cubic double perovskites as a promising class of materials to realize topological magnetic states, elucidates the likely stabilization mechanism of the triple-q state in these materials, and establishes neutron spectroscopy on powder samples as a valuable technique to distinguish multi-q from single-q structures, facilitating the discovery of topologically-nontrivial magnetic materials.

Presenters

  • Joe Paddison

    Oak Ridge National Lab, Oak Ridge National Laboratory

Authors

  • Joe Paddison

    Oak Ridge National Lab, Oak Ridge National Laboratory

  • Jiaqiang Yan

    Oak Ridge National Laboratory, Materials Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA

  • Hao Zhang

    University of Tennessee

  • Seunghwan Do

    Oak Ridge National Laboratory

  • Shang Gao

    Oak Ridge National Laboratory, Department of Physics, University of Science and Technology of China

  • Matthew B Stone

    Oak Ridge National Lab, Oak Ridge National Laboratory

  • David A Dahlbom

    University of Tennessee, University of Tennessee, Knoxville

  • Kipton M Barros

    Los Alamos Natl Lab, Theoretical Division and CNLS, Los Alamos National Laboratory

  • Cristian Batista

    University of Tennessee, University of Tennessee, Knoxville

  • Andy Christianson

    Oak Ridge National Laboratory, Oak Ridge National Lab