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Revealing Emergent Magnetic Charge in a Topological Antiferromagnet with Diamond Quantum Magnetometry

ORAL

Abstract

Whirling topological textures play a key role in exotic phases of magnetic materials and offer promise for logic and memory applications. In antiferromagnets, these textures exhibit enhanced stability and faster dynamics with respect to ferromagnetic counterparts, but they are also difficult to observe due to their vanishing net magnetic moment. Diamond quantum magnetometry offers a promising route to image such weak features through its high sensitivity and vectorial field detection. Here, we image the topological textures in the archetypal antiferromagnet, hematite, and reveal that these textures host in parallel a rich tapestry of monopolar, dipolar and quadrupolar magnetic charge distributions. By extracting field orientations, we demonstrate direct readout of the previously inaccessible antiferromagnetic vorticity, which is connected to magnetic charge through a duality relation. Our work highlights the critical role that diamond quantum magnetometry could play in exploring emergent phenomena and topological spintronics in quantum materials.

(A.T., H.J., M.H. contributed equally)

Publication: A manuscript on this work is currently under review.<br><br>Our previous related studies:<br>1. Jani, H. et al. Antiferromagnetic half-skyrmions and bimerons at room temperature. Nature 590, 74 (2021).<br>2. Jani, H., et al. Reversible hydrogen control of antiferromagnetic anisotropy in a-Fe2O3. Nature Communications 12, 1668 (2021).<br>3. Lim, Z. S.,* Jani, H.,* Venkatesan, T. & Ariando, A. Skyrmionics in correlated oxides. MRS Bulletin 46, 1053 (2021).

Presenters

  • Hariom Jani

    University of Oxford

Authors

  • Hariom Jani

    University of Oxford

  • Anthony Tan

    Univ of Cambridge

  • Michael Hoegen

    University of Cambridge

  • Lucio Stefan

    Niels Bohr Institute

  • Claudio Castelnovo

    Univ of Cambridge, University of Cambridge

  • Daniel Braund

    University of Cambrdige

  • Alexandra Geim

    University of Cambridge

  • Matthew Feuer

    Univ of Cambridge

  • Helena S Knowles

    University of Cambridge

  • Ariando Ariando

    Natl Univ of Singapore

  • Paolo G Radaelli

    University of Oxford

  • Mete Atatüre

    Univ of Cambridge, University of Cambridge