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Large anomalous Nernst effect in canted antiferromagnet YbMnBi<sub>2</sub>

ORAL

Abstract

A large anomalous Nernst effect (ANE) is crucial for thermoelectric energy conversion applications because the associated unique transverse geometry facilitates module fabrication. Topological ferromagnets with large Berry curvatures show large ANEs; however, they face drawbacks such as strong magnetic disturbances and low mobility due to high magnetization. YbMnBi2, as a canted antiferromagnet, surprisingly shows a large ANE conductivity of ~10 A m−1 K−1 that surpasses large values observed in other ferromagnets (3–5 A m−1 K−1). The canted spin structure of Mn guarantees a non-zero Berry curvature, but generates only a weak magnetization three orders of magnitude lower than that of general ferromagnets. The heavy Bi with a large spin–orbit coupling enables a large ANE and low thermal conductivity, whereas its highly dispersive px/y orbitals ensure low resistivity. The high anomalous transverse thermoelectric performance and extremely small magnetization make YbMnBi2 an excellent candidate for transverse thermoelectrics.

Publication: Pan, Y., Le, C., He, B. et al. Giant anomalous Nernst signal in the antiferromagnet YbMnBi2. Nat. Mater. 21, 203–209 (2022). https://doi.org/10.1038/s41563-021-01149-2

Presenters

  • Yu Pan

    Max Planck Institute for Chemical Physics of Solids

Authors

  • Yu Pan

    Max Planck Institute for Chemical Physics of Solids

  • Congcong Le

    RIKEN

  • Bin He

    Max Planck Institute for Chemical Physics of Solids

  • Sarah J Watzman

    University Of Cincinnati

  • Mengyu Yao

    Max Planck Institute for Chemical Physics of Solids, Max-Planck-Institute for Chemical Physics of Solids

  • Johannes Gooth

    IBM Research - Zurich, University Bonn

  • Joseph P Heremans

    Ohio State University, The Ohio State University

  • Yan Sun

    Max Planck Institute for Chemical Physics of Solids

  • Claudia Felser

    Max Planck Institute for Chemical Physic, Max Planck Institute for Chemical Physics of Solids