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Spin-polarized imaging of strongly interacting fermions in the magnetic phases of Weyl candidate CeBi

ORAL · Invited

Abstract

CeBi has a rich magnetic phase diagram and several predicted topological states that vary with magnetic phase. Here we focus on the ferrimagnetic and fully-polarized phases of CeBi, where our density functional theory (DFT) calculations predict several Weyl nodes near the Fermi level (Ef). We use spin-polarized scanning tunneling microscopy (SP-STM) and spectroscopy to image the surface magnetic order, and quasiparticle interference (QPI) imaging to quantify the band splitting of the ferrimagnetic and fully polarized phases with respect to the ground antiferromagnetic phase. In the ferrimagnetic phase, strong suppression of the surface spin-polarization at Ef, coincident with a Fano line shape in dI/dV, suggests the Bi p states partially Kondo screen the f magnetic moments, and this p-f mixing causes strong Fermi-level band renormalization. The QPI measurements support p band flattening and ~100 meV splitting, suggesting a strongly interacting magnetic Weyl semimetal with robustly spaced Weyl nodes. In fully polarized CeBi, on the (001) surface we discover that the outer Bi 6p band splits by ~ 200 meV, which is large enough to overcome the hybridization gap and give rise to a magnetic Weyl state. Our SP-STM and QPI measurements in three magnetic phases of CeBi paint a consistent picture of a strongly interacting magnetic Weyl semimetal that can be driven between different topological phases with the external field.

Publication: 1. C. E. Matt, Y. Liu, H. Pirie, N. C. Drucker, N. H. Jo, B. Kuthanazhi, Z. Huang, C. Lane, J.-X. Zhu, P. C. Canfield, and J. E. Hoffman, Spin-polarized imaging of strongly interacting fermions in the ferrimagnetic state of the Weyl candidate CeBi, Physical Review B 105, 085134 (2022). <br>2. Measured band splitting supports Weyl nodes in fully polarized CeBi (in preparation)

Presenters

  • Yu Liu

    Harvard University

Authors

  • Yu Liu

    Harvard University

  • Christian E Matt

    Harvard University

  • Harris S Pirie

    Harvard University

  • Nathan C Drucker

    Harvard University

  • Robert-Jan Slager

    Univ of Cambridge, University of Cambridge

  • Na Hyun Jo

    Iowa State University

  • Brinda Kuthanazhi

    Iowa State University

  • Sergey L Budko

    Iowa State University, Ames National Laboratory/Iowa State University

  • Zhao Huang

    Los Alamos National Laboratory

  • Christopher A Lane

    Los Alamos National Laboratory

  • Jianxin Zhu

    Los Alamos Natl Lab, Los Alamos National Lab, Los Alamos National Laboratory

  • Paul C Canfield

    Iowa State University, Ames National Laboratory, Ames National Laboratory/Iowa State University

  • Jenny E Hoffman

    Harvard University