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Driven-dissipative electron transport in a quantized conducting array

ORAL

Abstract

Nanojunction experiments with single molecules or quantum dots placed between macroscopic leads allow the exploration of quantum transport at the nanoscale [1]. We study driven-dissipative electron transport in a quantized conducting array of coupled two-level electron sites with a Markovian quantum master equation approach [2] that includes Coulomb interactions, electron tunneling, radiative recombination and non-radiative thermal relaxation [2]. Using literature data [3], we reproduce experimental negative conductance results for a thynylene AH molecular junction at 6 K. By driving a conducting array with resonant incoherent light, photon-induced currents are produced at zero bias voltage, whose current direction depends on the degree of delocalization of the array electrons. Conditions for current-induced light generation are also discussed.

Publication: [1] M. Thoss and F. Evers, J. Chem. Phys. 148, 030901 (2018).<br>[2] F. Recabal and F. Herrera, submitted (2021).<br>[3] M. L. Perrin et al. Nat. Nanotechnol. 9, 830-834. (2014).

Presenters

  • Felipe A Recabal

    Univ de Santiago de Chile

Authors

  • Felipe A Recabal

    Univ de Santiago de Chile

  • Felipe Herrera

    Univ de Santiago de Chile