Quantum critical point and phase separation at finite doping in Hund metals.

ORAL

Abstract

"Hund metals”  are multi-orbital paramagnetic metals with sizeable effects due to the intra-atomic exchange energy or Hund’s coupling, and are characterised by strong, orbital-selective correlations and large fluctuating local magnetic moments. Their physics is relevant for iron-based superconductors and other materials like transition metal oxides.

A general feature found in models and realistic simulations of these materials, and corroborated by experimental data, is a frontier crossing the doping-interaction strength plane, and originating from the Mott transition point of the half-filled system, across which the aforementioned defining features are strongly enhanced.

This frontier is a cross-over at large doping while approaching half-filling it becomes a first-order transition between two metals. It features a phase separation zone ending in a quantum critical point at finite doping.

I will show that all this phenomenology is due to the first-order nature of the Mott transition and can be back-tracked to a small energy scale splitting the atomic ground-state multiplet, in this case the Hund’s coupling. 

I will highlight the perfect parallel with a leading scenario for the physics of the cuprates, and thus possibly a universal one for materials showing high-Tc superconductivity.

Publication: L. de' Medici, PRL 118, 167003 (2017)
M. Chatzieleftheriou et al. PRB 102, 205127 (2020)
T. Gorni et al. PRB 104, 014507 (2021)
P. Villar Arribi and L. de' Medici, PRB 104, 125130(2021)
M. Chatzieleftheriou, A. Kowalski, M. Berovic, A. Amaricci, M. Capone, L. De Leo, G. Sangiovanni and L. de' Medici (in preparation, 2021)

Presenters

  • Luca de' Medici

    ESPCI Paris

Authors

  • Luca de' Medici

    ESPCI Paris