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Toward understanding the depletion of two-level systems in glasses

ORAL

Abstract

 The density of Two-level systems (TLS)  controls the low-temperature thermal properties in glasses. It is recently found that TLS are almost depleted in ultrastable glasses. Although it is thought to have a close relationship with the dramatic decrease of quasi-localized modes (QLMs), it is not yet clearly formalized.  Based on the soft-potential model and the tunneling TLS model, we argue that the TLS correspond to the QLMs with being a typical frequency ω0.  Their density n0  is proportional to the density of QLMs  DL0) and to the fraction of equal double-wells f(ω0) at ω0. We numerically estimate ω0 and n0 in computer glasses at different stabilities.  We find that ω0 is about  10% to 20% of the Debye frequency.   n0  decreases by a factor of 500 in ultrastable glasses than poorly prepared glasses with both DL0) and f(ω0) playing a significant role. Remarkably, the estimations of n0  are consistent with the order of magnitude of the change in n0 found in experiment in amorphous silicon. 

Presenters

  • Wencheng Ji

    Ecole Polytechnique Federale de Lausanne

Authors

  • Wencheng Ji

    Ecole Polytechnique Federale de Lausanne