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RKKY coupled local-moment magnetism in NaFe<sub>1-x</sub>Cu<sub>x</sub>As

ORAL

Abstract

Using high resolution 23Na NMR measurements on lightly Cu-doped metallic single crystals of NaFe1-xCuxAs (x ≈ 0.01) and numerical simulation, we present direct evidence of the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction in this pnictide system. The magnetic Cu2+ impurities are polarized by external field, inducing a spin polarization of the conduction electrons. Aided by computer simulation, we identify the 23Na NMR satellite resonances with the RKKY oscillations of this spin polarization coupled to loal moments at Fe sites via exchange interaction. Our 23Na spin-lattice and spin-spin relaxation data exhibits signature of an itinerant and inhomogeneous AFM phase in this system. Our NMR results indicate coexistence of local and itinerant magnetism in lightly Cu-doped NaFe1-xCuxAs.

Publication: Xin, Yizhou, et al., arXiv preprint arXiv:2107.04976v3 (2021)

Presenters

  • Yizhou Xin

    Northwestern University

Authors

  • Yizhou Xin

    Northwestern University

  • Ingrid Stolt

    Northwestern University

  • Zhai Gan

    Northwestern University

  • William P Halperin

    Northwestern University, Dept. Phys., Northwestern University

  • Yu Song

    Zhejiang University

  • Pengcheng Dai

    Rice Univ, Rice University

  • Chongde Cao

    Northwestern Polytechnical University