Correlated insulators, density wave states, and their nonlinear optical response in magic-angle twisted bilayer graphene

The correlated insulator (CI) states and the recently discovered density wave (DW) states in magic-angle twisted bilayer graphene (TBG) have stimulated intense research interest. However, up to date, the nature of these "featureless" correlated states observed at different integer and fractional fillings of the flat bands are still elusive, which are lack of direct experimental characters. Thus an experimental probe to identify the characters of these featureless CI and DW states are urgently needed. In this work, we theoretically study the correlated insulators and density wave states at different integer and fractional fillings of the flat bands in magic-angle TBG based on extended unrestricted Hartree-Fock calculations including the Coulomb screening effects from the remote bands. We further investigate the nonlinear optical responses, such as second-harmonic generations and shift-current responses, of the various correlated states, and find that the different components of the nonlinear optical conductivities can be used to identify the nature of these CI and DW states at most of the fillings. Thus we propose nonlinear optical response as a unique experimental probe to unveil the nature of the peculiar CI and DW states discovered in experiments in magic-angle TBG.