Modulating optical emission from dipolar excitons in vdW heterostructures by surface acoustic waves

Zach J Hadjri; Luka M Devenica; Sudipta Dubey; Weijie Li; Xin Lu; Takashi Taniguchi; Kenji Watanabe; Ajit Srivastava

Modulating optical emission from dipolar excitons in vdW heterostructures by surface acoustic waves

ORAL

Abstract

Surface acoustic waves (SAW) can couple to excitons via strain fields allowing for dynamic optoelectronics. Recently, interlayer excitons with permanent out-of-plane dipole moment have been discovered in transition metal dichalcogenide heterostructures. Due to their long lifetimes, interlayer excitons are expected to interact strongly with SAW. The strain field through deformation potential or piezoelectric coupling can create a dynamic localization for excitons. In order to analyze the effects of the SAW on the properties of excitons, we fabricated a device with a MoSe₂/WSe₂ heterobilayer on a LiNbO₃ substrate with interdigitated transducers to propagate SAW. Low temperature photoluminescence spectroscopy was used to characterize the system. We observe that the dipolar interlayer excitons couple to SAW and their optical emission is modulated accordingly.

March 16, 2022, 2:54 PM – March 16, 2022, 3:06 PM

Presenters

Zach J Hadjri

Emory University

Authors

Zach J Hadjri

Emory University
Luka M Devenica

Emory University
Sudipta Dubey

IIT Kanpur
Weijie Li

Emory University
Xin Lu

Tulane Univ
Takashi Taniguchi

National Institute for Materials Science, Tsukuba, Japan, National Institute for Materials Science, NIMS, Kyoto Univ, International Center for Materials Nanoarchitectonics, National Institute for Materials Science, 1-1 Namiki, Ibaraki 305-0044, Japan., 3 National Institute for Materials Science, Tsukuba, Japan, National Institute for Materials Science; 1-1 Namiki, Tsukuba, Ibaraki 305-0044, Japan, National Institute of Materials Science, Tsukuba, Japan, National Institute of Materials Science, Advanced Materials Laboratory, National Institute for Materials Science, 1-1 Namiki, Tsukuba, 305-0044, Japan, National Institute for Materials Science (Japan), International Center for Materials Nanoarchitectonics, National Institute for Materials Science, International Center for Materials Nanoarchitectonics, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan, Kyoto University, International Center for Materials Nanoarchitectonics, International Center for Materials Nanoarchitectonics, National Institute for Materials Science, Tsukuba, Japan, International Center for Materials Nanoarchitectonics, National Institute for Materials Science, Japan, International Center for Materials Nanoarchitectonics, National Institute for MaterialsScience, 1-1 Namiki, Tsukuba 305-0044, Japan, National Institute for Material Science, Japan, National Institute for Material Science, National Institute of Material Sciences, Japan, NIMS, Tsukuba, 2National Institute for Materials Science, Namiki 1-1, Ibaraki 305-0044, Japan., National Institute of Materials Science, Tsukuba, Ibaraki 305-0044, Japan, National Institute for Materials Science, Japan, International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science, 1-1 Namiki Tsukuba, Ibaraki 305-0044, Japan., NIMS, Japan, National Institute for Materials Science (NIMS), NIMS. Japan, International Center for Material Nanoarchitectonics, National Institute for Materials Science, Tsukuba, Japan, International Center for Material Nanoarchitectonics, National Institute for Materials Science, National Institute for Materials Science Tsukuba, National Institute for Materials Science, 1-1 Namiki, National Institute for Materials Science of Japan, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan, NIMS - National Institute for Material Science, Japan, International Center for Materials Nanoarchitectonics, National Institute for Material Science, Tsukuba, Ibaraki 305-0044, Japan., National Institute for Material Science, Tsukuba, National Institute for Materials Science, International Center for Materials Nanoarchitectonics, International Center for Materials Nanoarchitectonics, National Institute for Materials Science, 1-1 Namiki, Tsukuba, Ibaraki 305-0044, Japan, National Institute of Material Science, National Institute for Materials Science,1-1 Namiki, Tsukuba, 305-0044, Japan
Kenji Watanabe

National Institute for Materials Science, Tsukuba, Japan, National Institute for Materials Science, NIMS, Research Center for Functional Materials, National Institute for Materials Science, Tsukuba, Ibaraki 305-0044, Japan, Research Center for Functional Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan., Research Center for Functional Materials, National Institute for Materials Science, Advanced, Materials Laboratory, NIMS, 3 National Institute for Materials Science, Tsukuba, Japan, National Institute for Materials Science; 1-1 Namiki, Tsukuba, Ibaraki 305-0044, Japan, National Institute of Materials Science, Tsukuba, Japan, National Institute of Materials Science, Advanced Materials Laboratory, National Institute for Materials Science, 1-1 Namiki, Tsukuba, 305-0044, Japan, National Institute for Materials Science (Japan), National Institute for Materials Science, Japan, Research Center for Functional Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan, Research Center for Functional Materials, Research Center for Functional Materials, National Institute for Materials Science, Tsukuba, Japan, Research Center for Functional Materials, National Institute for Materials Science, Japan, Research Center for Functional Materials, National Institute for Materials Science, 1-1Namiki, Tsukuba 305-0044, Japan, National Institute for Material Science, Japan, National Institute for Material Science, National Institute of Material Sciences, Japan, NIMS, Tsukuba, 2National Institute for Materials Science, Namiki 1-1, Ibaraki 305-0044, Japan., National Institute of Materials Science, Tsukuba, Ibaraki 305-0044, Japan, National Institute for Materials Science Japan, NIMS, Japan, nims, National Institute for Materials Science, Research Center for Functional Materials, Japan, National Institute for Materials Science Tsukuba, National Institute for Materials Science, 1-1 Namiki, National Institute for Materials Science of Japan, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan, NIMS - National Institute for Material Science, Japan, Research Center for Functional Materials, National Institute for Material Science, Tsukuba, Ibaraki, 305-0044, Japan., National Institute for Material Science, Tsukuba, National Institute for Materials Science, Tsukuba, Ibaraki 305-0044, Japan, National Institute for Materials Science (NIMS), National Institute for Materials Science, Research Center for Functional Materials, Research Center for Functional Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba, Ibaraki 305-0044, Japan, National Institute of Material Science, Kyoto Univ, National Institute for Materials Science,1-1 Namiki, Tsukuba, 305-0044, Japan
Ajit Srivastava

Emory University