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Polaronic behavior in La<sub>1.2</sub>Sr<sub>1.8</sub>Mn<sub>2</sub>O<sub>7</sub>

ORAL

Abstract

La1.2Sr1.8Mn2O7 has been an intriguing candidate for probing electronic correlations due to the concomitant emergence of colossal magneto resistance with its paramagnetic-insulating to ferromagnetic-metallic transition at Tc = 120 K. Experimental evidence has demonstrated the relevance of polarons across the phase transition. In particular, early ARPES studies showed the abrupt formation of a small quasi-particle peak with strong mass renormalization in the metal phase which has been associated with a polaronic metal state. Yet, conflicting results revealing finite quasi particle spectral weight even above Tc and combined ARPES/STM studies showing sensitivity to the cleaved surface cast doubt on the polaronic metal scenario. Here we use resonant inelastic X-ray scattering (RIXS) which is a bulk-sensitive two-photon-probe. In contrast to ARPES which measures the single particle spectral function, RIXS probes collective excitations and is thus especially suitable for the investigation of charge-lattice coupled phenomena. In this presentation, we will discuss the RIXS signatures of polarons in La1.2Sr1.8Mn2O7.

Presenters

  • Daniel Jost

    Stanford University, SLAC - Natl Accelerator Lab

Authors

  • Daniel Jost

    Stanford University, SLAC - Natl Accelerator Lab

  • Matteo Rossi

    SLAC - Natl Accelerator Lab

  • Yonghun Lee

    Stanford University

  • John F Mitchell

    Argonne National Laboratory

  • Amol Singh

    Natl Synchrotron Rad Res Ctr

  • Hsiaoyu Huang

    Natl Synchrotron Rad Res Ctr, National Synchrotron Radiation Research Center

  • Di-Jing Huang

    Natl Synchrotron Rad Res Ctr

  • Zhixun Shen

    Stanford University, Geballe Laboratory for Advanced Materials, Stanford University, USA, Stanford Univ

  • Thomas P Devereaux

    Stanford Univ, Stanford University; SLAC National Accelerator Laboratory, Stanford University

  • Wei-Sheng Lee

    SLAC - Natl Accelerator Lab