Polaronic behavior in La<sub>1.2</sub>Sr<sub>1.8</sub>Mn<sub>2</sub>O<sub>7</sub>
ORAL
Abstract
La1.2Sr1.8Mn2O7 has been an intriguing candidate for probing electronic correlations due to the concomitant emergence of colossal magneto resistance with its paramagnetic-insulating to ferromagnetic-metallic transition at Tc = 120 K. Experimental evidence has demonstrated the relevance of polarons across the phase transition. In particular, early ARPES studies showed the abrupt formation of a small quasi-particle peak with strong mass renormalization in the metal phase which has been associated with a polaronic metal state. Yet, conflicting results revealing finite quasi particle spectral weight even above Tc and combined ARPES/STM studies showing sensitivity to the cleaved surface cast doubt on the polaronic metal scenario. Here we use resonant inelastic X-ray scattering (RIXS) which is a bulk-sensitive two-photon-probe. In contrast to ARPES which measures the single particle spectral function, RIXS probes collective excitations and is thus especially suitable for the investigation of charge-lattice coupled phenomena. In this presentation, we will discuss the RIXS signatures of polarons in La1.2Sr1.8Mn2O7.
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Presenters
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Daniel Jost
Stanford University, SLAC - Natl Accelerator Lab
Authors
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Daniel Jost
Stanford University, SLAC - Natl Accelerator Lab
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Matteo Rossi
SLAC - Natl Accelerator Lab
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Yonghun Lee
Stanford University
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John F Mitchell
Argonne National Laboratory
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Amol Singh
Natl Synchrotron Rad Res Ctr
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Hsiaoyu Huang
Natl Synchrotron Rad Res Ctr, National Synchrotron Radiation Research Center
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Di-Jing Huang
Natl Synchrotron Rad Res Ctr
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Zhixun Shen
Stanford University, Geballe Laboratory for Advanced Materials, Stanford University, USA, Stanford Univ
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Thomas P Devereaux
Stanford Univ, Stanford University; SLAC National Accelerator Laboratory, Stanford University
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Wei-Sheng Lee
SLAC - Natl Accelerator Lab