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Twist-angle controls interlayer exciton lifetimes in MoSe<sub>2</sub>/WSe<sub>2</sub> heterostructures

ORAL

Abstract

We investigate the twist angle dependent interlayer exciton lifetimes in MoSe2/WSe2 twisted bilayers (TBLs) capsulated by hexagonal boron nitride (hBN). Three R-stacking style samples with different twist angles are prepared with careful angle alignment and measured by time-resolved photoluminescence at low-temperature. The interlayer exciton lifetimes are found to change significantly with a small change in the twist angle by one order of magnitude. Using a low-energy continuum model, we theoretically explain two possible mechanisms influencing twist angle dependent interlayer exciton radiative lifetimes. The shift to indirect transitions in the momentum space with an increasing twist angle and the energy modulation from the moiré potential both have a significant impact on interlayer exciton lifetimes. We further predict distinct temperature dependence of interlayer exciton lifetimes in TBLs with different twist angles, which is partially validated by experiments.

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Presenters

  • Junho Choi

    University of Texas at Austin, Department of Physics, The University of Texas at Austin

Authors

  • Junho Choi

    University of Texas at Austin, Department of Physics, The University of Texas at Austin

  • Matthias Florian

    Institute for Theoretical Physics, University of Bremen

  • Alexander Steinhoff-List

    Institute for Theoretical Physics, University of Bremen

  • Daniel Erben

    Institute for Theoretical Physics, University of Bremen

  • Kha Tran

    University of Texas at Austin, Department of Physics, The University of Texas at Austin, United States Naval Research Laboratory

  • Dong Seob Kim

    University of Texas at Austin, Department of Physics, The University of Texas at Austin

  • Liuyang Sun

    Department of Physics, The University of Texas at Austin

  • Jiamin Quan

    University of Texas at Austin, Department of Physics, The University of Texas at Austin, Department of Physics, Center of Complex Quantum Systems, University of Texas at Austin

  • Rob Claassen

    Department of Physics, The University of Texas at Austin

  • Somak Majumder

    Los Alamos National Laboratory

  • Jennifer A Hollingsworth

    Center for Integrated Nanotechnologies, Materials, Physics, and Applications Division, Los Alamos National Laboratory, Los Alamos National Laboratory, Center for Integrated Nanotechnologies, Los Alamos National Laboratory

  • Takashi Taniguchi

    National Institute for Materials Science, National Institute for Materials Science, Japan, National Institure for Materials Science, Advanced Materials Laboratory, National Institute for Materials Science, NIMS, National Institute of Materials Science, National Institute for Materials Science (NIMS), International Center for Materials Nanoarchitectonics, National Institute for Materials Science, National Institute for Materials Science,1-1 Namiki, National Institute of Material Science, National Institute for Materials Science, Tsukuba, Japan, International Center for Materials Nanoarchitectonics, NIMS, Research Center for Functional Materials, National Institute for Materials Science, National Institute of Materials Science, Tsukuba, Japan, National Institude for Materials Science, International Center for Materials Nanoarchitectonics, National Institute for Materials Science, Tsukuba 305-0044, Japan, International Center for Materials Nanoarchitectonics, National Institute for Materials, NIMS - Japan, National Institute for Materials Science ,Japan, National Institute for Materials Science, Tsukuba, 305-0044, Ibaraki, Japan, National Institute for Material Science, National Institute for Material Science, 1-1 Namiki, Tsukuba 305-0044, Japan, National Institute for Material Science Japan, 8International Center for Materials Nanoarchitectonics, NIMS Tsukuba, National Institute for Materials Science: Namiki, Tsukuba, Ibaraki, JP, National Institue for Material Science, National Institute for Materials Science,1-1 Namiki, Tsukuba, 305-0044, Japan, Research Center for Functional Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan, Research Center for Functional Materials, National In, Research Center for Functional Materials, Japan, Research Center for Functional Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba, 305-0044, Japan, International Center for Material Nanoarchitectonics, National Institute for Materials Science, International Center for Materials Nanoarchitectonics, NIMS Suguba, NIMS, Tsukuba, Japan, National Cheng Kung University, National Institute for Materials Science, Namiki 1-1, Tsukuba, 305-0044, Ibaraki, Japan, National institute of material science, Advanced Materials Laboratory, National Institute for Materials Science, 1-1 Namiki, Tsukuba, 305-0044, Japan, Advanced Materials Laboratory, NIMS, National Institute for Materials Science, International Center for Materials Nanoarchitectonics, National Institute of Material Science, Japan, Tsukuba, National Institute for Materials Science

  • Kenji Watanabe

    National Institute for Materials Science, National Institute for Materials Science, Japan, National Institure for Materials Science, Advanced Materials Laboratory, National Institute for Materials Science, NIMS, National Institute of Materials Science, National Institute for Materials Science (NIMS), Research Center for Functional Materials, National Institute for Materials Science, National Institute for Materials Science,1-1 Namiki, National Institute of Material Science, National Institute for Materials Science, Tsukuba, Japan, Research Center for Functional Materials, NIMS, National Institute of Materials Science, Tsukuba, Japan, National Institude for Materials Science, National Institute for Materials Science, Tsukuba, Ibaraki, Japan, Research Center for Functional Materials, National Institute for Materials Science, Tsukuba 305-0044, Japan, International Center for Materials Nanoarchitectonics, National Institute for Materials, NIMS - Japan, National Institute for Materials Science ,Japan, National Institute for Materials Science, Tsukuba, 305-0044, Ibaraki, Japan, National Institute for Material Science, National Institute for Material Science, 1-1 Namiki, Tsukuba 305-0044, Japan, National Institute for Material Science Japan, NIMS Tsukuba, National Institute for Materials Science, Research Center for Functional Materials, Japan, Research Center for Functional Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan, National Institute for Materials Science: Namiki, Tsukuba, Ibaraki, JP, National Institue for Material Science, National Institute for Materials Science,1-1 Namiki, Tsukuba, 305-0044, Japan, Materials, NIMS, Research Center for Functional Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan, Research Center for Functional Materials, National In, Research Center for Functional Materials, Japan, International Center for Materials Nanoarchitectonics, National Institute for Materials Science, International Center for Materials nanoarchtectonics, National Institute for Materials Science, 1-1 Namiki, Tsukuba, 305-0044, Japan, NIMS Suguba, NIMS, Tsukuba, Japan, National Institute for Materials Science, Namiki 1-1, Tsukuba, 305-0044, Ibaraki, Japan, National institute of material science, Advanced Materials Laboratory, National Institute for Materials Science, 1-1 Namiki, Tsukuba, 305-0044, Japan, Advanced Materials Laboratory, NIMS, Research Center for Functional Materials, National Institute for Materials Science, Ibaraki, Japan, National Institute for Materials Science, Research Center for Functional Materials, National Institute of Material Science, Japan, Tsukuba, National Institute for Materials Science

  • Keiji Ueno

    Chemistry, Saitama University, Department of Chemistry, Saitama University

  • Akshay K Singh

    Department of Physics, Indian Institute of Science

  • Galan Moody

    University of California, Santa Barbara, Department of Electrical and Computer Engineering, University of California Santa Barbara

  • Frank Jahnke

    Institute for Theoretical Physics, University of Bremen

  • Xiaoqin (Elaine) Li

    University of Texas at Austin, Physics, University of Texas at Austin, Department of Physics, University of Texas at Austin, U.T. Austin, Department of Physics, The University of Texas at Austin, Department of Physics, Center of Complex Quantum Systems, University of Texas at Austin