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Singular charge fluctuations at a magnetic quantum critical point

Invited

Abstract

The heavy fermion compound YbRh2Si2 is well known for its large fan of linear-in-temperature “strange metal” resistivity emerging from a quantum critical point at the border of antiferromagnetic order. Previous studies revealed properties [1] that are beyond the description of the Landau framework of order parameter fluctuations, and compatible with a Kondo destruction quantum critical point [2]. Here, we probed the charge dynamics of this system by performing terahertz time-domain transmission spectroscopy experiments on high-quality YbRh2Si2 thin films grown by molecular beam epitaxy. We observe frequency over temperature scaling of the optical conductivity, with a critical exponent close to 1 in agreement with the linear-in-temperature dc resistivity, over a wide temperature and frequency range [3]. This dynamical scaling proves that charge carriers are a central ingredient to the singular physics at the border of antiferromagnetic order, and therefore strongly underpins the Kondo destruction nature of the observed quantum criticality.

[1] S. Paschen, T. Lühmann, S. Wirth, P. Gegenwart, O. Trovarelli, C. Geibel, F. Steglich, P. Coleman, and Q. Si, Nature 432, 881 (2004); S. Friedemann, N. Oeschler, S. Wirth, C. Krellner, C. Geibel, F. Steglich, S. Paschen, S. Kirchner, and Q. Si, Proc. Natl. Acad. Sci. USA 107, 14547 (2010).
[2] Q. Si, S. Rabello, K. Ingersent, and J. L. Smith, Nature 413, 804 (2001); P. Coleman, C. Pepin, Q. Si, and R. Ramazashvili, J. Phys. Condens. Matter 13, R723 (2001); T. Senthil, M. Vojta, and S. Sachdev, Phys. Rev. B 69, 035111 (2004).
[3] L. Prochaska, X. Li, D.C. MacFarland, A.M. Andrews, M. Bonta, E.F. Bianco, S. Yazdi, W. Schrenk, H. Detz, A. Limbeck, Q. Si, E. Ringe, G. Strasser, J. Kono, and S. Paschen, Science 367, 285 (2020).

Presenters

  • Lukas Prochaska

    Vienna Univ of Technology

Authors

  • Lukas Prochaska

    Vienna Univ of Technology

  • Xinwei Li

    Rice University, Department of Physics, California Institute of Technology, Department of Electrical and Computer Engineering, Rice University

  • Don MacFarland

    Vienna Univ of Technology

  • Aaron Maxwell Andrews

    Vienna Univ of Technology

  • Maximilian Bonta

    Vienna Univ of Technology

  • Elisabeth Bianco

    Rice University

  • Sadegh Yazdi

    Rice University

  • Werner Schrenk

    Vienna Univ of Technology

  • Hermann Detz

    Vienna Univ of Technology

  • Andreas Limbeck

    Vienna Univ of Technology

  • Qimiao Si

    Rice Univ, Physics and Astronomy, Rice university, Rice University, Department of Physics and Astronomy, Rice University, Department of Physics & Astronomy, Rice Center for Quantum Materials, Rice University, Houston, Texas 77005, USA

  • Emilie Ringe

    Rice University

  • Junichiro Kono

    Electrical and Computer Engineering, Rice University, Department of Electrical and Computer Engineering, Rice Univ, Rice University, Rice Univ, Department of Electrical and Computer Engineering, Rice University, Department of Physics and Astronomy, Rice University

  • Gottfried Strasser

    Vienna Univ of Technology

  • Silke Buehler-Paschen

    Institute of Solid State Physics, Vienna University of Technology, Vienna Univ of Technology