Coherence protection and decay mechanism in qubit ensembles under concatenated continuous driving

Dense ensembles of spin qubits are valuable for quantum applications, even though their coherence protection remains challenging. Continuous dynamical decoupling can protect ensemble qubits from noise while allowing gate operations, but it is hindered by the additional noise introduced by the driving. Concatenated continuous driving (CCD) techniques can, in principle, mitigate this problem. We experimentally demonstrate the improved control by simultaneously addressing a dense Nitrogen-vacancy (NV) ensemble with 10^10 spins. We achieve an experimental 15-fold improvement in coherence time for an arbitrary, unknown state, and a 500-fold improvement for an arbitrary, known state, corresponding to driving the sidebands and the center band of the resulting Mollow triplet, respectively. By extending the generalized Bloch equation approach to the CCD scenario, we identify the noise sources that dominate the decay mechanisms in NV ensembles, confirm our model by experimental results, and identify the driving strengths yielding optimal coherence. Our results can be directly used to optimize qubit coherence protection under continuous driving and bath driving, and enable applications in robust pulse design and quantum sensing.