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Moiré metrology of energy landscapes in van der Waals heterostructures

ORAL

Abstract

The emerging field of twistronics has revolutionized quantum materials research. At the small twist limit, and particularly under strain, as atomic relaxation prevails, the emergent moiré superlattice encodes elusive insights into the local interlayer interaction. In this work we introduce moiré metrology as a combined experiment-theory framework to probe the stacking energy landscape of bilayer structures at the 0.1 meV/atom scale, outperforming the gold-standard of quantum chemistry. Through studying the shapes of moiré domains with numerous nano-imaging techniques, and correlating with multi-scale modelling, we assess and refine first-principle models for the interlayer interaction. We document the prowess of moiré metrology for three representative twisted systems: bilayer graphene, double bilayer graphene and H-stacked MoSe2/WSe2. Moiré metrology establishes sought after experimental benchmarks for interlayer interaction, thus enabling accurate modelling of twisted multilayers.

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Presenters

  • Dorri Halbertal

    Columbia University, Columbia Univ, Physics, Columbia University

Authors

  • Dorri Halbertal

    Columbia University, Columbia Univ, Physics, Columbia University

  • Nathan Finney

    Columbia University, Mechanical Engineering, Columbia University

  • Sai Sunku

    Columbia University, Columbia Univ, Physics, Columbia University

  • Alexander Kerelsky

    Physics, Columbia University

  • Carmen Rubio Verdú

    Department of Physics, Columbia University, New York, New York 10027, USA, Columbia University, Physics, Columbia University

  • Sara Shabani

    Physics, Columbia University, Columbia Univ, Columbia University

  • Lede Xian

    Max Planck Institute

  • Stephen Carr

    Harvard University, Brown University, Department of Physics, Brown University, Physics, Brown University

  • Shaowen Chen

    Columbia Univ, Physics, Columbia University

  • Charles Zhang

    University of California, Santa Barbara, Physics, Columbia University

  • Lei Wang

    Physics, Nanjing University, Columbia University, Physics, Columbia University, Cornell University

  • Derick Gonzalez-Acevedo

    Columbia Univ, Physics, Columbia University

  • Alexander McLeod

    Columbia University, Department of Physics, Columbia University, Columbia Univ, Physics, Columbia University

  • Daniel Rhodes

    Physics, University of Wisconsin - Madison, Physics, Columbia University, Materials Science and Engineering, University of Wisconsin-Madison, University of Wisconsin-Madison

  • Kenji Watanabe

    National Institute for Materials Science, National Institute for Materials Science, Japan, National Institure for Materials Science, Advanced Materials Laboratory, National Institute for Materials Science, NIMS, National Institute of Materials Science, National Institute for Materials Science (NIMS), Research Center for Functional Materials, National Institute for Materials Science, National Institute for Materials Science,1-1 Namiki, National Institute of Material Science, National Institute for Materials Science, Tsukuba, Japan, Research Center for Functional Materials, NIMS, National Institute of Materials Science, Tsukuba, Japan, National Institude for Materials Science, National Institute for Materials Science, Tsukuba, Ibaraki, Japan, Research Center for Functional Materials, National Institute for Materials Science, Tsukuba 305-0044, Japan, International Center for Materials Nanoarchitectonics, National Institute for Materials, NIMS - Japan, National Institute for Materials Science ,Japan, National Institute for Materials Science, Tsukuba, 305-0044, Ibaraki, Japan, National Institute for Material Science, National Institute for Material Science, 1-1 Namiki, Tsukuba 305-0044, Japan, National Institute for Material Science Japan, NIMS Tsukuba, National Institute for Materials Science, Research Center for Functional Materials, Japan, Research Center for Functional Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan, National Institute for Materials Science: Namiki, Tsukuba, Ibaraki, JP, National Institue for Material Science, National Institute for Materials Science,1-1 Namiki, Tsukuba, 305-0044, Japan, Materials, NIMS, Research Center for Functional Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan, Research Center for Functional Materials, National In, Research Center for Functional Materials, Japan, International Center for Materials Nanoarchitectonics, National Institute for Materials Science, International Center for Materials nanoarchtectonics, National Institute for Materials Science, 1-1 Namiki, Tsukuba, 305-0044, Japan, NIMS Suguba, NIMS, Tsukuba, Japan, National Institute for Materials Science, Namiki 1-1, Tsukuba, 305-0044, Ibaraki, Japan, National institute of material science, Advanced Materials Laboratory, National Institute for Materials Science, 1-1 Namiki, Tsukuba, 305-0044, Japan, Advanced Materials Laboratory, NIMS, Research Center for Functional Materials, National Institute for Materials Science, Ibaraki, Japan, National Institute for Materials Science, Research Center for Functional Materials, National Institute of Material Science, Japan, Tsukuba, National Institute for Materials Science

  • Takashi Taniguchi

    National Institute for Materials Science, National Institute for Materials Science, Japan, National Institure for Materials Science, Advanced Materials Laboratory, National Institute for Materials Science, NIMS, National Institute of Materials Science, National Institute for Materials Science (NIMS), International Center for Materials Nanoarchitectonics, National Institute for Materials Science, National Institute for Materials Science,1-1 Namiki, National Institute of Material Science, National Institute for Materials Science, Tsukuba, Japan, International Center for Materials Nanoarchitectonics, NIMS, Research Center for Functional Materials, National Institute for Materials Science, National Institute of Materials Science, Tsukuba, Japan, National Institude for Materials Science, International Center for Materials Nanoarchitectonics, National Institute for Materials Science, Tsukuba 305-0044, Japan, International Center for Materials Nanoarchitectonics, National Institute for Materials, NIMS - Japan, National Institute for Materials Science ,Japan, National Institute for Materials Science, Tsukuba, 305-0044, Ibaraki, Japan, National Institute for Material Science, National Institute for Material Science, 1-1 Namiki, Tsukuba 305-0044, Japan, National Institute for Material Science Japan, 8International Center for Materials Nanoarchitectonics, NIMS Tsukuba, National Institute for Materials Science: Namiki, Tsukuba, Ibaraki, JP, National Institue for Material Science, National Institute for Materials Science,1-1 Namiki, Tsukuba, 305-0044, Japan, Research Center for Functional Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan, Research Center for Functional Materials, National In, Research Center for Functional Materials, Japan, Research Center for Functional Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba, 305-0044, Japan, International Center for Material Nanoarchitectonics, National Institute for Materials Science, International Center for Materials Nanoarchitectonics, NIMS Suguba, NIMS, Tsukuba, Japan, National Cheng Kung University, National Institute for Materials Science, Namiki 1-1, Tsukuba, 305-0044, Ibaraki, Japan, National institute of material science, Advanced Materials Laboratory, National Institute for Materials Science, 1-1 Namiki, Tsukuba, 305-0044, Japan, Advanced Materials Laboratory, NIMS, National Institute for Materials Science, International Center for Materials Nanoarchitectonics, National Institute of Material Science, Japan, Tsukuba, National Institute for Materials Science

  • Efthimios Kaxiras

    Harvard University, Department of Physics, Harvard University, Physics, Harvard University

  • Cory Dean

    Columbia University, Department of Physics, Columbia University, Physics, Columbia University, Columbia Univ

  • James Hone

    Columbia Univ, Columbia University, Department of Mechanical Engineering, Columbia University, Mechanical Engineering, Columbia University

  • Abhay Narayan

    Department of Physics, Columbia University, Physics, Columbia University, Columbia Univ, Department of Physics, Columbia University, New York, New York 10027, USA, Columbia University

  • Dante Kennes

    Institut fur Theorie der Statistischen Physik, RWTH Aachen, RWTH Aachen University, Institut für Theorie der Statistischen Physik, RWTH Aachen University, Institute for Theory of Statistical Physics, Aachen University, RWTH Aachen, Aachen, Institute for Theory of Statistical Physics, RWTH Aachen University

  • Angel Rubio

    Max Plank Institute for the Structure and Dynamics of Matter; Center for Computational Quantum Physics Flatiron Institute, Max Planck Institute for the Structure and Dynamics of Matter, Theory, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Inst Structure & Dynamics of Matter, Physics, Max Planck Institute, Max Planck Institute for Structure and Dynamics of Matter and Center for Free-Electron Laser Science, Max Planck Institute for the Structure and Dynamics of Matter, Center for Free Electron Laser Science, 22761 Hamburg, Germany, Max Planck Institute for the Structure and Dynamics of Matter and Center Free-Electron Laser Science, Hamburg, Germany, Max Planck Institute for the Structure and Dynamics of Matter, Hamburg, Germany, MPSD Hamburg, Max Planck Institute, Max Planck Inst Structure & Dynamics of Matter; Center for Computational Quantum Physics Flatiron Institute, Simons Foundation NY, USA, Theory, Max Planck Inst Structure & Dynamics of Matter

  • Dmitri Basov

    Columbia University, Department of Physics, Columbia University, Physics, Columbia University, Columbia Univ