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Unraveling the Morphological Evolutions during Solvent Vapor Annealing for Organic Solar Cells Using in situ Resonant Soft X-Ray Scattering

POSTER

Abstract

Solvent vapor annealing (SVA) is one of the most effective pre-electrode deposition techniques, which has been applied in many efficient organic solar cells. In current research, we used a customized in situ multimodal system to reveal the dynamics of phase separation inside the bulk-heterojunction thin films during SVA via resonant soft x-ray scattering (RSoXS). Solvent-vapor-induced molecular crystallization is of importance to provide the driving force of the domain generation and evolution processes. However, with the introduction of solvent vapor for a long time, coarsening of the film appeared at the film surface, which led to the deteriorating of the device performances. These results indicated that in situ RSoXS is a quite useful technique to bridge the gap to understand the relationship of film growth mechanisms and device efficiency.

Presenters

  • Wenkai Zhong

    Lawrence Berkeley National Laboratory

Authors

  • Wenkai Zhong

    Lawrence Berkeley National Laboratory

  • Isvar Cordova

    Lawrence Berkeley National Laboratory, MSD, Lawrence Berkeley National Lab

  • Yufeng Jiang

    University of California, Berkeley, Lawrence Berkeley National Laboratory

  • Cheng Wang

    Lawrence Berkeley National Laboratory, ALS, Lawrence Berkeley National Lab

  • Feng Liu

    Shanghai Jiaotong University

  • Thomas Russell

    Univ of Mass - Amherst, Polymer Science and Engineering, University of Massachusetts Amherst, Lawrence Berkeley National Laboratory, Polymer Science and Engineering Department, UMass