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Switching 2D Magnetic States via Pressure Tuning of Layer Stacking

ORAL

Abstract

The physical properties of two-dimensional van der Waals crystals can be sensitive to the interlayer coupling. For 2D magnets, theory suggests that the interlayer exchange coupling strongly depends on layer separation, while the stacking arrangement can even change the sign of the interlayer magnetic exchange, thus drastically modifying the ground state. Here, we demonstrate pressure tuning of magnetic order in the 2D magnet CrI3. We probe the magnetic states using tunneling and scanning magnetic circular dichroism microscopy measurements. We find that the critical field for the spin-flip transition can be more than doubled by hydrostatic pressure. In bilayer CrI3, pressure induces a transition from layered antiferromagnetic to ferromagnetic phases. In trilayer CrI3, pressure can create coexisting domains of three phases, one ferromagnetic and two antiferromagnetic. The observed changes in magnetic order can be explained by changes in the stacking arrangement. Such coupling between stacking order and magnetism provides ample opportunities for designer magnetic phases and functionalities.

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Presenters

  • Tiancheng Song

    University of Washington

Authors

  • Tiancheng Song

    University of Washington

  • Zaiyao Fei

    University of Washington, Physics, University of Washington

  • Matthew A Yankowitz

    Physics, Columbia University, Columbia University, University of Washington, Columbia Univ

  • Zhong Lin

    University of Washington

  • Qianni Jiang

    University of Washington

  • Kyle Hwangbo

    University of Washington

  • Qi Zhang

    University of Washington, Advanced Photon Source, Argonne National Laboratory

  • Bosong Sun

    University of Washington

  • Takashi Taniguchi

    National Institute for Materials Science, Japan, National Institute for Material Science, National Institute for Materials Science, National Institute for Materials Science, Tsukuba, Research Center for Functional Materials, NIMS, nims, Advanced Materials Laboratory, National Institute for Materials Science, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan, NIMS, National Institute for Material Science - Japan, NIMS Tsukuba, National Institute for Materials Science, Namiki 1-1, Ibaraki 305-0044, Japan., National Institute for Materials Science (NIMS), National Institute for Materials Science,Tsukuba, Ibaraki 305-0047, Japan, Advanced Materials Laboratory, NIMS, Japan, National Institute for Materials Science,1-1 Namiki, Tsukuba, 305-0044, Japan, National Institute of Materials Science, National Institute for Materials Science, University of Tsukuba, National Institute for Materials Science, Tsukuba, Japan, National Institue for Material Science, Tsukuba, Advanced Materials Laboratory, NIMS, Advanced Materials Laboratory, National Institute for Materials Science, Tsukuba 305-0044, Japan, Advanced Matrials Lab, NIMS, National Institute for Material Science, Tsukuba, Japan, National institute for materials science, NIMS-Tsukuba, NIMS, Japan, National Institute for Materials Science, Namiki Tsukuba Ibaraki, Japan, Advanced Materials Laboratory, National Institute for Materials Science, Tsukuba, Japan, NIMS Japan, National Institute for Materials Science, Tsukuba, Ibaraki 305-0044, Japan, Research Center for Functional Materials, National Institute for Materials Science, Tsukuba, Ibaraki, Japan, Advanced Materials Laboratory, National Institute of Materials Science, Advanced Materials Laboratory, National Institute for Materials Science 1-1 Namiki, Tsukuba, 305-0044, Japan, National Institute of Material Science, 1-1 Namiki, Tsukuba 305-0044, Japan, National Institute for Material Science (Japan), Physics, NIMS, National Institute of Materials Science, Japan, National Institute of Materials Science, Tsukuba, Ibaraki 305-0044, Japan, NIMS - Tsukuba

  • Kenji Watanabe

    National Institute for Materials Science, Japan, National Institute for Material Science, National Institute for Materials Science, National Institute for Materials Science, Tsukuba, Research Center for Functional Materials, NIMS, nims, Advanced Materials Laboratory, National Institute for Materials Science, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan, NIMS, National Institute for Material Science - Japan, NIMS Tsukuba, National Institute for Materials Science, Namiki 1-1, Ibaraki 305-0044, Japan., National Institute for Materials Science (NIMS), National Institute for Materials Science,Tsukuba, Ibaraki 305-0047, Japan, Advanced Materials Laboratory, NIMS, Japan, National Institute for Materials Science,1-1 Namiki, Tsukuba, 305-0044, Japan, National Institute of Materials Science, National Institute for Materials Science, University of Tsukuba, National Institute for Materials Science, Tsukuba, Japan, National Institute for Material Science, Japan, National Institue for Material Science, Tsukuba, Advanced Materials Laboratory, NIMS, Advanced Materials Laboratory, National Institute for Materials Science, Tsukuba 305-0044, Japan, Advanced Matrials Lab, NIMS, National Institute for Material Science, Tsukuba, Japan, National institute for materials science, NIMS-Tsukuba, NIMS, Japan, National Institute for Materials Science, Namiki Tsukuba Ibaraki, Japan, NIRM, Advanced Materials Laboratory, National Institute for Materials Science, Tsukuba, Japan, NIMS Japan, National Institute for Materials Science, Tsukuba, Ibaraki 305-0044, Japan, Research Center for Functional Materials, National Institute for Materials Science, Tsukuba, Ibaraki, Japan, Advanced Materials Laboratory, National Institute of Materials Science, Advanced Materials Laboratory, National Institute for Materials Science 1-1 Namiki, Tsukuba, 305-0044, Japan, National Institute of Material Science, 1-1 Namiki, Tsukuba 305-0044, Japan, National Institute for Material Science (Japan), Physics, NIMS, National Institute of Materials Science, Japan, National Institute of Materials Science (NIMS), National Institute of Materials Science, Tsukuba, Ibaraki 305-0044, Japan, NIMS - Tsukuba

  • Michael McGuire

    Oak Ridge National Laboratory, Materials Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge National Lab, Materials Science Division, Oak Ridge National Laboratory

  • David E Graf

    Florida State University, National High Magnetic Field Laboratory, Florida State University, Department of Physics, National High Magnetic Field Laboratory, Florida State University, Florida, USA, National High Magnetic Field Laboratory, National High Magnetic Field Lab, Florida State University, National High Magnetic Field Laboratory and Department of Physics, Florida State University, Florida State Univ, Natl High Magnetic Field Lab, National High Magnetic Field Lab, Tallahassee, FL 32310, USA, National High Magnetic Field Laboratory, 1800 E. Paul Dirac Drive, Tallahassee, FL 32310, USA, National High Magnetic Field Laboratory-Florida State University, National High Magnetic Field Laboratory, Tallahassee, FL, NHMFL, Florida State University, NHMFL

  • Ting Cao

    University of Washington, Department of Physics, University of California at Berkeley and Lawrence Berkeley National Laboratory, Physics, University of Washington, Department of Materials Science and Engineering, University of Washington and Geballe Laboratory for Advanced Materials, Stanford University

  • Jiun-Haw Chu

    University of Washington, Department of Physics, University of Washington, Physics, University of Washington

  • David Cobden

    University of Washington, Physics, University of Washington

  • Cory Dean

    Department of Physics, Columbia University, Columbia University, Columbia Univ, Physics, Columbia University

  • Di Xiao

    Physics, Carnegie Mellon University, Carnegie Mellon University, Carnegie Mellon Univ, Department of Physics, Carnegie Mellon University

  • Xiaodong Xu

    University of Washington, Physics, University of Washington