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Distinct magneto-Raman signatures of spin-flip phase transitions in CrI<sub>3</sub>

ORAL

Abstract

The discovery of 2-dimensional (2D) materials, such as CrI3, that retain magnetic ordering at monolayer thickness has resulted in a surge of research in 2D magnetism from both pure and applied perspectives. Here, we report a magneto-Raman spectroscopy study on multilayered CrI3, focusing on two new features in the spectra which appear at temperatures below the magnetic ordering temperature and were previously assigned to high frequency magnons. We observe a striking evolution of the Raman spectra with increasing magnetic field in which clear, sudden changes in intensities of the modes are attributed to the interlayer ordering changing from antiferromagnetic to ferromagnetic at a critical magnetic field. Our work highlights the sensitivity of the Raman modes to weak interlayer spin ordering in CrI3. In addition, we theoretically examine potential origins for the new modes, which we deduce are unlikely single magnons.

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Presenters

  • Amber McCreary

    National Institute of Standards and Technology, NIST

Authors

  • Amber McCreary

    National Institute of Standards and Technology, NIST

  • Thuc Mai

    NIST, National Institute of Standards and Technology

  • Franz Utermohlen

    Ohio State University

  • Jeffrey Simpson

    Towson Univ, Towson University, Physics, Towson University, Department of Physics, Towson University

  • Kevin Garrity

    National Institute of Standards and Technology, MML, NIST, Materials Measurement Lab, National Institute of Standards and Technology, NIST

  • Xiaozhou Feng

    Penn State University

  • Dmitry Shcherbakov

    Ohio State University, Ohio State Univ - Columbus

  • Yanglin Zhu

    Department of Physics, Pennsylvania State University, University Park, Pennsylvania 16802, USA, Physics, The Pennsylvania State University, Department of Physics, Pennsylvania State University, Pennsylvania State University, Penn State University, Physics, Penn State University, Pennsylvania state University

  • Jin Hu

    Univ of Arkansas-Fayetteville, Physics, Univ of Arkansas-Fayetteville, University of Arkansas

  • Daniel Weber

    Ohio State University, Ohio State Univ - Columbus

  • Kenji Watanabe

    National Institute for Materials Science, Japan, National Institute for Material Science, National Institute for Materials Science, National Institute for Materials Science, Tsukuba, Research Center for Functional Materials, NIMS, nims, Advanced Materials Laboratory, National Institute for Materials Science, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan, NIMS, National Institute for Material Science - Japan, NIMS Tsukuba, National Institute for Materials Science, Namiki 1-1, Ibaraki 305-0044, Japan., National Institute for Materials Science (NIMS), National Institute for Materials Science,Tsukuba, Ibaraki 305-0047, Japan, Advanced Materials Laboratory, NIMS, Japan, National Institute for Materials Science,1-1 Namiki, Tsukuba, 305-0044, Japan, National Institute of Materials Science, National Institute for Materials Science, University of Tsukuba, National Institute for Materials Science, Tsukuba, Japan, National Institute for Material Science, Japan, National Institue for Material Science, Tsukuba, Advanced Materials Laboratory, NIMS, Advanced Materials Laboratory, National Institute for Materials Science, Tsukuba 305-0044, Japan, Advanced Matrials Lab, NIMS, National Institute for Material Science, Tsukuba, Japan, National institute for materials science, NIMS-Tsukuba, NIMS, Japan, National Institute for Materials Science, Namiki Tsukuba Ibaraki, Japan, NIRM, Advanced Materials Laboratory, National Institute for Materials Science, Tsukuba, Japan, NIMS Japan, National Institute for Materials Science, Tsukuba, Ibaraki 305-0044, Japan, Research Center for Functional Materials, National Institute for Materials Science, Tsukuba, Ibaraki, Japan, Advanced Materials Laboratory, National Institute of Materials Science, Advanced Materials Laboratory, National Institute for Materials Science 1-1 Namiki, Tsukuba, 305-0044, Japan, National Institute of Material Science, 1-1 Namiki, Tsukuba 305-0044, Japan, National Institute for Material Science (Japan), Physics, NIMS, National Institute of Materials Science, Japan, National Institute of Materials Science (NIMS), National Institute of Materials Science, Tsukuba, Ibaraki 305-0044, Japan, NIMS - Tsukuba

  • Takashi Taniguchi

    National Institute for Materials Science, Japan, National Institute for Material Science, National Institute for Materials Science, National Institute for Materials Science, Tsukuba, Research Center for Functional Materials, NIMS, nims, Advanced Materials Laboratory, National Institute for Materials Science, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan, NIMS, National Institute for Material Science - Japan, NIMS Tsukuba, National Institute for Materials Science, Namiki 1-1, Ibaraki 305-0044, Japan., National Institute for Materials Science (NIMS), National Institute for Materials Science,Tsukuba, Ibaraki 305-0047, Japan, Advanced Materials Laboratory, NIMS, Japan, National Institute for Materials Science,1-1 Namiki, Tsukuba, 305-0044, Japan, National Institute of Materials Science, National Institute for Materials Science, University of Tsukuba, National Institute for Materials Science, Tsukuba, Japan, National Institue for Material Science, Tsukuba, Advanced Materials Laboratory, NIMS, Advanced Materials Laboratory, National Institute for Materials Science, Tsukuba 305-0044, Japan, Advanced Matrials Lab, NIMS, National Institute for Material Science, Tsukuba, Japan, National institute for materials science, NIMS-Tsukuba, NIMS, Japan, National Institute for Materials Science, Namiki Tsukuba Ibaraki, Japan, Advanced Materials Laboratory, National Institute for Materials Science, Tsukuba, Japan, NIMS Japan, National Institute for Materials Science, Tsukuba, Ibaraki 305-0044, Japan, Research Center for Functional Materials, National Institute for Materials Science, Tsukuba, Ibaraki, Japan, Advanced Materials Laboratory, National Institute of Materials Science, Advanced Materials Laboratory, National Institute for Materials Science 1-1 Namiki, Tsukuba, 305-0044, Japan, National Institute of Material Science, 1-1 Namiki, Tsukuba 305-0044, Japan, National Institute for Material Science (Japan), Physics, NIMS, National Institute of Materials Science, Japan, National Institute of Materials Science, Tsukuba, Ibaraki 305-0044, Japan, NIMS - Tsukuba

  • Joshua Goldberger

    Ohio State Univ - Columbus, Ohio State University, Chemistry, The Ohio State University

  • Zhiqiang Mao

    Pennsylvania State University, Tulane University, Physics, Pennsylvania State University, Department of Physics, Pennsylvania State University, University Park, Pennsylvania 16802, USA, Physics, The Pennsylvania State University, Department of Physics, Pennsylvania State University, Penn State University, Physics, Penn State University, The Pennsylvania State University

  • Chun Ning Lau

    Ohio State University, Department of Physics, The Ohio State University, Deparment of Physics, The Ohio State University, Ohio State Univ - Columbus

  • Yuanming Lu

    Ohio State University

  • Nandini Trivedi

    Department of Physics, Ohio State Univ - Columbus, Physics, The Ohio State University, The Ohio State University, Ohio State Univ Columbus, Ohio State University, Ohio State Univ - Columbus, Physics, Ohio State University

  • Rolando Valdes Aguilar

    Ohio State Univ - Columbus, Ohio State Univ, Physics, The Ohio State University, Ohio State University, Department of Physics, The Ohio State University

  • Angela Hight Walker

    National Institute of Standards and Technology, NIST, National Institute of Standards and Technology (NIST)