Weak crystallization of fluctuating skyrmion textures in MnSi

We report an experimental study of the emergence of non-trivial topological winding and long-range order across the paramagnetic to skyrmion lattice (SkL) transition in the transition metal helimagnet MnSi. Combining measurements of the susceptibility with small angle neutron scattering, neutron resonance spin echo spectroscopy and all-electrical microwave spectroscopy, we find evidence of skyrmion textures in the paramagnetic state exceeding 10³ Å with lifetimes above several 10^-9 s. Our experimental findings establish that the paramagnetic to SkL transition in MnSi is well-described by the Landau soft-mode mechanism of weak crystallization, originally proposed in the context of the liquid to crystal transition. As a key aspect of this theoretical model, the modulation-vectors of periodic small amplitude components of the magnetization form triangles that add to zero. In excellent agreement with our experimental findings, these triangles of the modulation-vectors entail the presence of the non-trivial topological winding of skyrmions already in the paramagnetic state of MnSi when approaching the SkL transition.
J. Kindervater et al., Phys. Rev. X (accepted for publication)