Spin waves and magnetic exchange interactions in the spin-ladder compounds BaFe$_{\mathrm{2}}$S$_{\mathrm{3}}$ and RbFe$_{\mathrm{2}}$Se$_{\mathrm{3}}$.

ORAL

Abstract

We report inelastic neutron scattering studies on the spin waves of BaFe$_{\mathrm{2}}$S$_{\mathrm{3}}$ and RbFe$_{\mathrm{2}}$Se$_{\mathrm{3}}$. Both of them exhibit similar stripe antiferromagnetic (AF) orders as that of BaFe$_{\mathrm{2}}$As$_{\mathrm{2}}$. At ambient pressure BaFe$_{\mathrm{2}}$S$_{\mathrm{3}}$ can be viewed as the parent state of the superconductivity discovered under pressure. Fitting the spin wave spectra to a Heisenberg Hamiltonian reveals a strong ferromagnetic (FM) exchange interaction (SJ$_{\mathrm{R}}$\textasciitilde 71 meV) along the rung direction, an AF SJ$_{\mathrm{L}}$\textasciitilde 49 meV along the leg direction, and a FM SJ$_{\mathrm{2}}$\textasciitilde 15 meV along the diagonal direction. The results are in clear contrast to the exchange interactions of the parent compounds of the other iron-based superconductors, suggesting that specific relative values for the exchange interactions do not appear to be unique for the parent states of the superconducting materials. However, identical measurements for insulating RbFe$_{\mathrm{2}}$Se$_{\mathrm{3}}$ reveal comparable exchange interactions as that of BaFe$_{\mathrm{2}}$As$_{\mathrm{2}}$, indicating the irrelevance of the fermiology for the existence of the stripe AF order among various Fe-based materials. arXiv:1609.00465, PRB 94,041111(R)(2016).

Authors

  • Meng Wang

    Sun Yat-Sen University

  • S. J. Jin

    Sun Yat-Sen University

  • Dao-Xin Yao

    Sun Yat-Sen University

  • Ming Yi

    Univ of California - Berkeley, University of California, Berkeley

  • Dunghai Lee

    University of California, Berkeley, Department of Physics, University of California, Berkeley; Materials Science Division, Lawrence Berkeley National Laboratories,

  • Robert Birgeneau

    University of California, Berkeley, UC Berkeley, University of California Berkeley

  • Hongchen Jiang

    SLAC National Accelerator Laboratory, Stanford Institute for Materials and Energy Sciences, SLAC, Stanford Institute for Materials and Energy Sciences

  • Yu Song

    Rice University

  • W. L. Zhang

    Institute of Physics, CAS

  • Huiqian Luo

    Institute of Physics, CAS, Institute of Physics (CAS)

  • H. L. Sun

    Institute of High Energy Physics, CAS

  • Andrew Christianson

    Oak Ridge National Laboratory, The Oak Ridge National Laboratory, Quantum Condensed Matter Division, Oak Ridge National Laboratory

  • Clarina dela Cruz

    Oak Ridge National Laboratory

  • Edith Bourret

    Lawrence Berkeley National Laboratory, Lawrence Berkeley National Laboratory, Berkeley, CA