How do ultrathin sheets attach to a fluid-fluid interface?

ORAL

Abstract

Thin elastic sheets when placed at the interface between immiscible fluids can lower the surface energy and hence act as surface active agents. Here we report experimental studies on the dynamics of attachment of ultrathin sheets to a fluid-fluid interface. A polymer film (thickness, t$=$30 to 500nm, and lateral size, W $\sim$ 1cm) is released in one of the liquid phases and driven towards the interface by gravity. At the interface, a slow initial nucleation process is followed by a rapid adsorption to the surface. Surprisingly, the three phase contact line remains stationary in the lab frame during most of the process, with the sheet bending sharply in the vicinity of the contact line. In the late stages of attachment, the sheet bends towards the interface and the contact line is observed to be moving. We find that at early times the attachment proceeds at a constant speed and compare this speed with scaling estimates.

Authors

  • Deepak Kumar

    University of Massachusetts Amherst, Univ of Mass - Amherst

  • Joseph D. Paulsen

    Syracuse University

  • Thomas Russell

    University of Massachusetts Amherst, University of Massachusetts, Amherst, Univ of Mass - Amherst, University of Massachusetts Amherst, Lawrence Berkeley National Lab, Univ. of Massachusetts Amherst

  • Benny Davidovich

    University of Massachusetts Amherst, UMass Amherst, University of Massachusetts, Amherst

  • Dominic Vella

    University of Oxford, Mathematical Institute, University of Oxford, Woodstock Rd, Oxford, OX2 6GG, Oxford University

  • Narayanan Menon

    University of Massachusetts Amherst, Univ of Mass - Amherst, TIFR Centre for Interdisciplinary Sciences, 21 Brundavan Colony, Osman Sagar Road, Narsingi, Hyderabad 500 075