Valley addressable exciton-polaritons in atomically thin MoSe$_2$

ORAL

Abstract

While conventional semiconductor technology relies on the manipulation of electrical charge for the implementation of computational logic, additional degrees of freedom such as spin offer alternative avenues for the encoding of information. In TMD monolayers, where spin-valley locking is present, strong retention of valley chirality has been reported for MoS$_2$, WSe$_2$ and WS$_2$ while MoSe$_2$ shows low polarization retention. Here, we show that by placing monolayers of MoSe$_2$ in an optical microcavity in the strong light-matter coupling regime, the valley polarization is regained with an enhancement of up to 7X compared with the bare monolayer. Here, polaritons introduce a fast relaxation mechanism which inhibits full valley spin relaxation of reservoir excitons due to the Maialle-Sham mechanism and allows for increased retention of polarization. A dynamical model reproduces the detuning dependence through the incorporation of cavity-modified exciton relaxation, allowing an estimate of the spin relaxation which is an order of magnitude faster than those reported in other TMDs. The valley addressability demonstrates the prospect of valleytronic devices based upon MoSe$_2$ embedded in photonic structures.

Authors

  • Scott Dufferwiel

    University of Sheffield

  • T. P. Lyons

    University of Sheffield

  • D. D. Solynshkov

    Blaise Pascal University

  • A. A. P. Trichet

    University of Oxford

  • F. Withers

    University of Manchester

  • S. Schwarz

    University of Sheffield

  • G. Malpuech

    Blaise Pascal University

  • J. M. Smith

    University of Oxford

  • K. S. Novoselov

    University of Manchester

  • M. S. Skolnick

    University of Sheffield

  • D. N. Krizhanovskii

    University of Sheffield

  • A. I. Tartakovskii

    University of Sheffield