Observation of interacting polaronic gas behavior in Ta-doped TiO$_{2}$ thin films via terahertz time-domain spectroscopy

ORAL

Abstract

Using terahertz time-domain spectroscopy (THz-TDS), we obtained the complex optical conductivity [$\tilde{\sigma} (\omega)$] of Ta-doped TiO$_{2}$ thin films --- a transparent conducting oxide (TCO), in the frequency range 0.3--2.7~THz, temperature range 10--300~K and various Ta dopings. Our results reveal the existence of an interacting polaronic gas in these TCOs, and suggest that their large conductivity is caused by the combined effects of large carrier density \textit{and} small electron-phonon coupling constant due to Ta doping.

Authors

  • Elbert Chia

    Nanyang Technological Univ

  • Liang Cheng

    Nanyang Technological Univ

  • James Lourembam

    Nanyang Technological Univ

  • S. G. Wu

    Nanyang Technological Univ

  • Mallikarjuna R. Motapothula

    National Univ Singapore

  • Tarapada Sarkar

    Center for Nanophysics \& Advanced Materials, University of Maryland, College Park, Maryland 20742, USA., National Univ Singapore

  • Venky Venkatesan

    National University of Singapore, National Univ Singapore