1D spin chain of Cu$^{2+}$ in Sr$_3$CuPtO$_6$ with possible Haldane physics

ORAL

Abstract

Antiferromagnetic spin chain systems have attracted considerable attention since the discovery of fractional spinon excitations in spin-half chain systems and Haldane gap phases in spin-one chain systems. It has been reported from bulk susceptibility and heat capacity measurements that the magnetic Cu$^{2+}$ ions in Sr$_3$CuPtO$_6$ exhibit S=1/2 Heisenberg spin chain behavior with a substantial amount of AFM interchain coupling. Using the modern time-of-flight inelastic neutron scattering spectrometer SEQUOIA at the SNS, we have probed the magnetic excitation spectrum for a polycrystalline sample of Sr$_3$CuPtO$_6$. Modeling with linear spin wave theory accounts for the major features of the spinwave spectra, including a nondispersive intense magnon band at 8meV. The magnetic excitations broaden considerably as temperature is increased, persisting up to above 100K and displaying a broad transition as previously seen in the susceptibility data. No spin gap is observed in the dispersive spin excitations at low momentum transfer, which we argue is consistent with Haldane physics in an ideal uniform S=1/2 spin-chain system.

Authors

  • Jonathan Leiner

    Seoul National University

  • Joosung Oh

    Center for Correlated Electron Systems, Institute for Basic Science, Seoul National University

  • Alexander Kolesnikov

    Oak Ridge National Laboratory, Oak Ridge National Lab

  • Matthew Stone

    ORNL, Oak Ridge National Laboratory, Quantum Condensed Matter Division, Oak Ridge National Laboratory

  • Manh Duc Le

    ISIS Facility, Rutherford Appleton Laboratory

  • Sang-Wook Cheong

    Rutgers University, Rutgers, The State University of New Jersey, Rutgers Univ, Rutgers Univ.

  • Je-Geun Park

    Seoul National University