Magnetic Phase Diagram of $\alpha$-RuCl$_3$

ORAL

Abstract

The layered honeycomb material $\alpha$-RuCl$_3$ is thought to possess unusual magnetic interactions including a strong bond-dependent Kitaev term, offering a potential opportunity to study a material near a well understood spin liquid phase. Although this material orders magnetically at low temperatures and is thus not a realization of a Kitaev spin liquid, it does show a broad continuum of magnetic excitations reminiscent of that expected for the spin liquid phase. It has also been proposed that a magnetic field could destabilize the magnetic order in this material and induce a transition into a spin liquid phase. Low temperature magnetization and specific heat measurements in this material have suggested a complex magnetic phase diagram with multiple unidentified magnetic phases present at low temperature. This has provided motivation for our work characterizing the magnetic transitions and phase diagram in $\alpha$-RuCl$_3$. I will present detailed bulk measurements combined with magnetic neutron diffraction measurements to map out the phase diagram and identify the various phases present.

Authors

  • Jennifer Sears

    University of Toronto

  • Young-June Kim

    University of Toronto

  • Yang Zhao

    NIST Center for Neutron Research

  • Jeffrey Lynn

    NIST Center for Neutron Research