Hidden Order in Spin-Liquid Gd$_3$Ga$_5$O$_{12}$
ORAL
Abstract
Frustrated magnetic materials are promising candidates for new states of matter because lattice geometry suppresses conventional magnetic dipole order, potentially allowing non-dipole (``hidden") order to emerge in its place. However, an atomic-scale model of a hidden-order state has been difficult to obtain because microscopic probes are not directly sensitive to hidden order. We use a combination of neutron-scattering experiments and reverse Monte Carlo refinements to develop a model of the spin-liquid state in the canonical frustrated magnet Gd$_3$Ga$_5$O$_{12}$. We show that this state exhibits a hidden order which has three unusual properties. First, it is a collective phenomenon, in which multipoles are formed from ten-spin loops. Second, it is long-range, with a diverging correlation length. Third, it is a consequence of the interplay between antiferromagnetic spin correlations and local planar magnetic anisotropy, which allows it to be indirectly observed in our neutron-scattering experiments.
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Authors
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Joseph Paddison
School of Physics, Georgia Institute of Technology, USA, and Department of Chemistry, University of Oxford, UK, and STFC-ISIS, UK
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Henrik Jacobsen
Nanoscience Center, University of Copenhagen, Denmark, and European Spallation Source, Sweden
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Oleg Petrenko
Department of Physics, University of Warwick, UK
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Maria Teresa Fern\'{a}ndez-D\'{i}az
Institut Max von Laue - Paul Langevin, France
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Pascale Deen
Nanoscience Center, University of Copenhagen, Denmark, and European Spallation Source, Sweden
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Andrew Goodwin
Department of Chemistry, University of Oxford, UK