Dynamics of the Ho$^{+3}$ magnetism in the multiferroic compound HoMnO$_3$ investigated via time domain terahertz spectroscopy

ORAL

Abstract

The multiferroic insulator HoMnO$_3$ possesses a diverse array of magnetism due to both magnetically active Mn$^{+3}$ and Ho$^{+3}$ moments, the latter of which sit at two distinct sites within its non-inversion symmetric hexagonal crystal structure. While previous studies have focused on the ordering of the Mn$^{+3}$ moments, little is known about the magnetic structure below $5$K where it is believed that there is at least partial ordering of the Ho$^{+3}$ ions. In principle, magnetic exchange interactions exist between both distinct Ho$^{+3}$ and Mn$^{+3}$ ions, resulting in an complex phase diagram with as many as five distinct phases found below T $=5$K and H $=3$T. While previous infrared studies have focused on the Ho$^{+3}$ crystal field levels, the spin excitations in the low frequency end of the far infrared remain unknown. We report the finding of new infrared absorptions via time domain terahertz spectroscopy which we attribute to the Ho$^{+3}$ moments. The corresponding field dependence is studied.

Authors

  • N.P. Armitage

    Johns Hopkins University

  • N. J. Laurita

    Johns Hopkins University, Johns Hopkins Univ

  • Rongwei Hu

    Rutgers University

  • Sang-Wook Cheong

    Rutgers, The State University of New Jersey, Rutgers University, Rutgers Center for Emergent Materials and Department of Physics and Astronomy, Rutgers University, Piscataway, New Jersey 08854, USA, RCEM, Rutgers Univ, Rutgers Univ, Department of Physics \& Astronomy, Rutgers University