In Situ Thin Film Growth and Characterization of Topological Dirac Semimetal Na$_3$Bi

ORAL

Abstract

The alkali pnictide Na$_3$Bi is a three-dimensional Dirac semimetal possessing Dirac-like dispersions in k$_x$, k$_y$ and k$_z$, that has attracted recent interest as a condensed matter system for realizing the chiral anomaly [1]. The high reactivity of sodium makes conventional synthesis and characterization extremely difficult: we circumvent this issue by combining thin film growth with low temperature STM and magnetotransport in one comprehensive UHV system. We have successfully grown Na$_3$Bi on $\alpha$-Al$_2$O$_3$ (0001) substrates, achieving low temperature mobilites in excess of 3,500 cm$^2$/Vs and carrier densities as low as 5 $\times$ 10 $^{12}$ cm$^{-2}$. Perpendicular magnetoresistance up to 1T shows quadratic behavior with weak anti-localization at low field. Quantitative analysis of this data suggests that our samples are in a charge inhomogeneous regime reminiscent of charge puddling in graphene [2]. [1] Xiong et. al Science (2015) doi:10.1126/science.aac6089 [2] Ramakrishnan et. al arXiv:1501.03815 (2015)

Authors

  • Jack Hellerstedt

    Monash Centre for Atomically Thin Materials

  • Mark Edmonds

    Monash Centre for Atomically Thin Materials

  • Chang Liu

    Monash Centre for Atomically Thin Materials

  • Navneeth Ramakrishnan

    NUS Singapore, Center for Advanced 2D Materials

  • Shaffique Adam

    Yale-NUS College, 16 College Avenue West, Singapore 138527, Singapore, Centre for Advanced 2D Materials and Department of Physics, National University of Singapore and Yale-NUS College, Yale-NUS College

  • Michael Fuhrer

    Monash Centre for Atomically Thin Materials, Monash University