The first single atom magnet

ORAL

Abstract

The prime feature of a magnet is to retain a significant fraction of its saturation magnetization in the absence of an external magnetic field. Realizing magnetic remanence in a single atom would allow storing and processing information in the smallest unit of matter. Here we show that individual rare-earth atoms on ultrathin insulating layers grown on non-magnetic metal substrates exhibit magnetic remanence and, therefore, are the first magnets formed by a single surface adsorbed atom. These magnets have a magnetic lifetime of 1500 s and a coercive field of 3.7 T at 10 K. In addition, their hysteresis loop remains open up to 30 K. This first example of a single atom magnet shows bistability at a temperature which is significantly higher than the best single molecule magnets reported so far. Its extraordinary stability is achieved by a suitable combination of magnetic ground state and adsorption site symmetry, and by decoupling the $4f$ spin from the underlying metal by a tunnel barrier.

Authors

  • Fabio Donati

    Ecole Polytechnique F\'{e}d\'{e}rale de Lausanne

  • Stefano Rusponi

    Ecole Polytechnique F\'{e}d\'{e}rale de Lausanne

  • Christian W\"{a}ckerlin

    Ecole Polytechnique F\'{e}d\'{e}rale de Lausanne

  • Aparajita Singha

    Ecole Polytechnique F\'{e}d\'{e}rale de Lausanne

  • Romana Baltic

    Ecole Polytechnique F\'{e}d\'{e}rale de Lausanne

  • Katharina Diller

    Ecole Polytechnique F\'{e}d\'{e}rale de Lausanne

  • Fran\c{c}ois Patthey

    Ecole Polytechnique F\'{e}d\'{e}rale de Lausanne

  • Edgar Fernandes

    Ecole Polytechnique F\'{e}d\'{e}rale de Lausanne

  • Harald Brune

    Ecole Polytechnique F\'{e}d\'{e}rale de Lausanne

  • Jan Dreiser

    Paul Scherrer Institute

  • Zeljko Sljivancanin

    Vin\v{c}a Institute of Nuclear Sciences

  • Kurt Kummer

    European Synchrotron Radiation Facility

  • Sebastian Stepanow

    ETH Z\"{u}rich

  • Luca Persichetti

    ETH Z\"{u}rich

  • Corneliu Nistor

    ETH Z\"{u}rich

  • Pietro Gambardella

    ETH Z\"{u}rich