The phase diagram of Sr$_{\mathrm{1-x}}$Na$_{\mathrm{x}}$Fe$_{2}$As$_{2}$: evidence of magnetic C4 phase universality

ORAL

Abstract

Determination of the nature of superconductivity in the high Tc iron based superconductors requires understanding the material's magnetic behavior out of which superconductivity arises. The apparent competition between superconductivity and magnetism in these materials and the appearance of superconductivity upon suppression of magnetism suggests magnetic fluctuations as a possible superconducting pairing mechanism. A recent study of the sodium doped barium 122 system which established the existence of a new magnetic phase formed within the AFM dome and its coexistence with superconductivity, has generated intense interest in the nature of this novel magnetic phase and given new insights to the driving force behind the magnetic transitions and preceding nematic fluctuations in this system. To search for evidence of a universality to this new magnetic and tetragonal C4 phase in the hole doped iron pnictides, polycrystalline Sr$_{\mathrm{1-x}}$Na$_{\mathrm{x}}$Fe$_{2}$As$_{2}$ samples were synthesized for measurements with x-ray and neutron diffraction experiments. In this talk, I will present results that show a more robust magnetic C4 phase, with a higher ordering temperature and stability over a larger range of compositions than has been seen in the Ba$_{\mathrm{1-x}}$Na$_{\mathrm{x}}$Fe$_{2}$As$_{2}$ counterparts.

Authors

  • Keith Taddei

    Northern Illinois University, Materials Science Division, Argonne National Laboratory

  • Jared Allred

    Argonne National Laboratory (ANL), Materials Science Division, Argonne National Laboratory, Argonne National Laboratory, Argonne Natl Lab

  • D.E. Bugaris

    ANL

  • Matthew Krogstad

    Northern Illinois University, Materials Science Division, Argonne National Laboratory

  • Stephan Rosenkranz

    ANL, Materials Science Division, Argonne National Laboratory

  • Raymond Osborn

    Argonne National Laboratory, ANL, Materials Science Division, Argonne National Laboratory

  • Helmut Claus

    ANL, Materials Science Division, Argonne National Laboratory

  • Duck-Young Chung

    ANL, Materials Science Division, Argonne National Laboratory

  • S.H. Lapidus

    ANL Advanced Photon Source

  • Mercouri Kanatzidis

    ANL and Northwestern University, Department of Chemistry, Northwestern University

  • Omar Chmaissem

    Northern Illinois University, DeKalb IL and Argonne National Laboratory, Argonne IL, ANL and Northern Illinois University, Northern Illinois University, Argonne National Laboratory