Nematic charge fluctuations and electron-phonon coupling in EuFe$_{2}$As$_{2}$ and SrFe$_{2}$As$_{2}$

ORAL

Abstract

We study phononic and electronic Raman scattering in the 122 iron pnictide parent compounds EuFe$_{2}$As$_{2}$ and SrFe$_{2}$As$_{2}$. Using polarized Raman spectra we identify all four Raman active phonon modes through the temperature range of 5-300 K from \textit{ab} plane and \textit{ac} plane. Strong interference of the phonon and the electronic continuum is observed in the A$_{g}$ channel below the tetragonal (D$_{4h}$) to orthorhombic (D$_{2h}$) (T-O) phase transition. Quasi-elastic Raman scattering induced by nematic fluctuations observed in the B$_{2g}$ channel in a wide temperature range above the T-O transition. The temperature dependence of the static Raman susceptibility derived from the Raman response $\chi'(0)= \frac{1}{\pi}P\int^{\infty}_{-\infty}\frac{\chi''(\omega)}{\omega}d\omega$ follows a Curie-Weiss like law A(T-T$_{0}$)$^{-1}$, where T$_{0}$ is about 50K below the T-O transition temperature. WLZ acknowledges ICAM support (NSF-IMI grant DMR-0844115), GB, VT and HHK acknowledge support by NSF DMR-1104884 and by U.S. DOE, BES, Award DE-SC0005463, AS acknowledges the support by US DOE, BES, Materials Sciences and Engineering Division.

Authors

  • Wei-Lu Zhang

    Chinese Academy of Sci (CAS), Rutgers, the State University of New Jersey, Rutgers, The State University of New Jersey

  • Verner Thorsmolle

    Rutgers, the State University of New Jersey, Rutgers, The State University of New Jersey

  • Hsiang-Hsi Kung

    Rutgers, the State University of New Jersey, Rutgers University

  • Philip Lubik

    Rutgers, the State University of New Jersey

  • Alexander Lee

    Rutgers, the State University of New Jersey

  • Girsh Blumberg

    Rutgers, the State University of New Jersey, Rutgers, The State University of New Jersey, Rutgers University

  • Pierre Richard

    Chinese Academy of Sci (CAS)

  • Hong Ding

    Chinese Academy of Sci (CAS), Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences

  • A.S. Sefat

    Oak Ridge National Laboratory, Oak Ridge National Lab, Materials Science and Technology Division, Oak Ridge National Laboratory

  • Jack Gillett

    Cavendish Laboratory, Cambridge University

  • Suchitra Sebastian

    Cavendish Laboratory, Cambridge University, University of Cambridge