Imaging electronic hot spots in the spectral function of the actinide UCoGa$_5$

ORAL

Abstract

We performed self-consistent GW-like calculations within the intermediate Coulomb-U coupling regime to investigate dynamic correlation effects in the intermetallic actinide UCoGa$_5$. This material is often used to contrast anomalous behavior in other U-115 and Pu-115 compounds, because it is presumed to be a conventional Fermi liquid that resembles a ``vegetable.'' First-principles electronic structure calculations were used as input, combined with the spin-fluctuation exchange approximation, to compute self-consistently the many-body self-energy responsible for dynamic correlation effects. We validated theory by angle-resolved photoemission spectroscopy (ARPES). The occurrence of electronic hot spots in the spectral function, accompanied by kinks and abrupt breaks in the slope of the quasiparticle dispersion were detected both at low (130 meV) and high (1 eV) binding energies below the Fermi energy. In conclusion, we found that dynamic correlation anomalies are adequately described by coupling between itinerant fermions and spin fluctuations arising from the particle-hole continuum of the spin-orbit-split 5f states of uranium.

Authors

  • Matthias J. Graf

    Los Alamos National Laboratory

  • T. Das

    Los Alamos National Laboratory, Theoretical Division, Los Alamos National Laboratory, Los Alamos Natl. Lab.

  • Tomasz Durakiewicz

    Los Alamos National Laboratory, MPA-CMMS Group, Los Alamos, NM 87544, USA, Los Alamos National Laboratory

  • Jian-Xin Zhu

    Los Alamos National Laboratory, Los Alamos, New Mexico 87545, Los Alamos National Laboratory, Theoretical Division, Los Alamos National Laboratory

  • John J. Joyce

    Los Alamos National Laboratory

  • John Sarrao

    Los Alamos National Laboratory