Covalent magnetic form factor and neutron scattering in cuprates

ORAL

Abstract

We investigate the effect of covalent hybridization on magnetic excitations measured by the inelastic neutron scattering (INS) in the 1D cuprate Sr$_2$CuO$_3$ and the 2D La$_2$CuO$_4$. It has been previously shown that strong hybridization of Cu 3d states with O p states leads to the dramatic modification of the measured INS intensity, which is strongly suppressed, by factor 2.5-3, compared to the ionic spin model [1]. The result was obtained by comparing the measured intensity in a chain cuprate Sr$_2$CuO$_3$ with the dynamical spin structure factor predicted by the exact theory [2] of the model spin-1/2 Heisenberg Hamiltonian, which is typically used for cuprates. In the present follow-up study we extend these measurements so as to probe directly the wave vector dependence of the magnetic form factor, which is the Fourier transform of the magnetic electron's density, both in Sr$_2$CuO$_3$, and in the LSCO parent material, the two-dimensional La$_2$CuO$_4$. Our results yield a model-independent measurement of the magnetic form factor and provide an explanation for the suppressed magnetic intensity in La$_2$CuO$_4$ and other cuprates.\\[4pt] [1] A. Walters, \emph{et. al}, Nature Physics {\bf 5}, 867 (2009).\\[0pt] [2] J.-S. Caux, R. Hagemans, J. Stat. Mech., {\bf P12013} (2006)

Authors

  • Igor Zaliznyak

    Brookhaven National Laboratory, Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory

  • Zhijun Xu

    Brookhaven National Laboratory, CMP\&MS Department, Brookhaven National Laboratory, Brookhaven National Lab

  • Genda Gu

    Brookhaven National Laboratory, CMP\&MS Department, Brookhaven National Laboratory, Condensed Matter Physics \& Materials Science Department, Brookhaven National Laboratory, Brookhaven National Laboratory, Upton, NY, Brookhaven National Laboratory, Condensed Matter Physics \& Materials Science Department, NY 11973, Brookheaven National Laboratory

  • Andrei T. Savici

    Oak Ridge National Laboratory, NSSD, Oak Ridge National Laboratory, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USA

  • Garrett E. Granroth

    Oak Ridge National Laboratory, Quantum Condensed Matter Division, Oak Ridge National Laboratory, NSSD, Oak Ridge National Laboratory

  • Matthew B. Stone

    Neutron Science Directorate, ORNL, NSSD, Oak Ridge National Laboratory, Quantum Condensed Matter Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USA