Mesoscale spin domain formation and their correlations in quasi-1D La$_{0.67}$Sr$_{0.33}$MnO$_3$ nanowires

ORAL

Abstract

Creating materials with nano-scale dimensions can introduce finite size and boundary effects, where the scale of the system boundaries near criticality becomes comparable to the correlation of competing orders in the material. To study these effects, we have fabricated arrays of quasi-1D nanowires from epitaxially grown La$_{0.67}$Sr$_{0.33}$MnO$_{3}$ (LSMO) thin films on SrTiO$_{3}$(STO) substrates. Our studies with resonant soft x-ray scattering (RSXS) reveal a non-trivial magnetic domain formation along different momentum directions in these wires. In addition, a new magnetic order was observed below 110K, likely induced by the STO structural transition. Below the Curie temperature we also observed a series of magnetic superlattice reflections, indicating collective mesoscale ordering of the magnetic moments into a pattern with a spatial period of five wires. Our calculations using dielectric susceptibility and Ising model simulations provide us an interpretation for the mechanism of domain formation and their long-range interaction through dipole coupling.

Authors

  • Xiaoqian M. Chen

    Frederick Seitz Materials Research Laboratory, University of Illinois at Urbana-Champaign

  • Nick Bronn

    Frederick Seitz Materials Research Laboratory, University of Illinois at Urbana-Champaign

  • Nadya Mason

    University of Illinois at Urbana-Champaign, Department of Physics and Materials Research Laboratory, University of Illinois at Urbana-Champaign, Frederick Seitz Materials Research Laboratory, University of Illinois at Urbana-Champaign

  • Peter Abbamonte

    University of Illinois Department of Physics, Frederick Seitz Materials Research Laboratory, University of Illinois at Urbana-Champaign

  • Jason Hoffman

    Argonne National Laboratory, Materials Science Division, Argonne National Lab

  • Anand Bhattacharya

    Argonne National Laboratory, Materials Science Division \& Center for Nanoscale Materials, Argonne National Lab, Argonne National Lab, Materials Science Division and Center for Nanoscale Materials, Argonne National Laboratory