Scanning Tunneling Microscopy and Spectroscopy of Fe[H$_2$B(Pz)$_2$]$_2$(bipy) Spin-Crossover Complex on Au(111)

ORAL

Abstract

Spin crossover compounds have externally-tunable magnetic moments that will be useful for spintronic applications if they result in correspondingly tunable electronic properties. In order to assess this electronic tunability, we have performed variable temperature scanning tunneling microscopy and spectroscopy on a known Fe(II) spin crossover compound, Fe[H$_2$B(Pz)$_2$]$_2$(bipy), thermally-evaporated onto a single crystal Au(111) surface. We report on the surface assembly of this molecule in few layer films including imaging with submolecular resolution. In addition, we use STS to probe the local density of electronic states across a temperature range spanning the low spin to high spin transition and compare with first principles electronic structure calculations.

Authors

  • Alex Pronschinske

    North Carolina State University

  • Geoff Lewis

    North Carolina State University

  • Yifeng Chen

    North Carolina State University, Department of Physics, North Carolina State University

  • Robert Bruce

    University of North Carolina

  • Wei You

    University of North Carolina

  • M. Buongiorno Nardelli

    North Carolina State University, Department of Physics, North Carolina State University, Department of Physics, North Carolina State University, Raleigh, NC 27695, NC State University, Raleigh and ORNL, Oak Ridge, TN

  • David Shultz

    North Carolina State University

  • Daniel B. Dougherty

    Department of Physics, North Carolina State University, North Carolina State University, Department of Physics, North Carolina State University, Raleigh, NC 27695