Magnetic non-uniformity in (La$_{0.4}$Pr$_{0.6})_{0.67}$Ca$_{0.33}$MnO$_{3}$ films and measurement of the strain-magnetization coupling coefficient

ORAL

Abstract

We have characterized the non-uniformity of chemical and magnetic properties of (La$_{0.4}$Pr$_{0.6})_{0.67}$Ca$_{0.33}$MnO$_{3}$ (LPCMO) films grown on NdGaO$_{3}$ using polarized neutron reflectometry (PNR). Our data indicate that the films exhibit coexistence of different magnetic phases as a function of depth. The variation of magnetism with depth is correlated with a variation of chemical composition with depth. Using PNR we also measured the magnetization depth profile of the LPCMO film as a function of applied bending stress. From these measurements we were able to obtain values for the coupling coefficients relating strain to the variation of the magnetization depth profile. Our results suggest that application of compressive (tensile) bending stress increases (suppresses) magnetization. We will discuss the implications of our results on the prevailing theories of the role of strain on phase separation in manganites.

Authors

  • S. Singh

    Los Alamos National Laboratory

  • M.R. Fitzsimmons

    Los Alamos National Laboratory, Los Alamos, NM 87545, Los Alamos National Laboratory

  • T. Lookman

    Los Alamos National Laboratory

  • Hyoungjeen Jeen

    Oak Ridge National Laboratory, Department of Physics, University of Florida

  • M.A. Roldan

    Complutense University, Madrid 28040, Spain

  • Maria Varela

    Condensed Matter Sciences Division Oak Ridge National Laboratory, Tennessee 37831-6031, USA, Oak Ridge National Laboratory, ORNL

  • Amlan Biswas

    Dept. Phys. and NHMFL, Univ. Florida, Department of Physics, University of Florida, University of Florida