Unusual interchain coupling effects in frustrated edge-shared chain cuprates with ferromagnetic NN in-chain coupling

ORAL

Abstract

We consider the effect of weak antiferromagnetic interchain coupling (AFM IC) on the saturation field, the magnetization curve, the phase diagram of multipolar phases at high magnetic fields, the dynamical magnetic structure factor, as well as the pitch angle at ambient fields applying the DMRG-technique to clusters of coupled long chains and the hard-core boson method to quasi-1D spin nematics at T=0 The critical AFM IC couplings for various multipolar phases and types of IC are determined. The results are applied to Li$_{2}$CuO$_{2}$, LiVCuO$_{4}$, Ca$_{2}$Y$_{2}$Cu$_{5}$O$_{10}$, as well as to linarite. The multipolar phases can be stabilized by easy-axis spin anisotropy. Linarite and LiVCuO$_{4}$, are found to be good candidates for the detection of mulipolar phases. Microscopic considerations based on the extended five-band Hubbard model and L(S)DA+$U $calculations provide exchange integrals which support the empirically found values for the main exchange integrals. We discuss the applicability of spin-wave theory and the role of quantum fluctuations for a correct description of magnetic excitations. Cases when a weak IC coupling dominates solely or predominantly the saturation field and/or the pitch angle are emphasized.

Authors

  • Stefan-Ludwig Drechsler

    IFW-Dresden, Institute of Theoretical Solid State Physics, Dresden, Germany

  • Satoshi Nishimoto

    IFW-Dresden, Institute of Theoretical Solid State Physics, Dresden, Germany, IFW Dresden, Germany

  • Jeroen van den Brink

    IFW Dresden, IFW-Dresden, Institute of Theoretical Solid State Physics, Dresden, Germany, IFW Dresden, Germany

  • Jiri Malek

    IFW-Dresden, Institute of Theoretical Solid State Physics, Dresden, Germany

  • Roman Kuzian

    Institute of Material Sciences NASU, Ukraine, Kiev

  • Johannes Richter

    University of Magdeburg, Germany

  • Miriam Schmitt

    MPI-CPFS, Dresden, Germany

  • Helge Rosner

    MPI CPfS Dresden, MPI-CPFS, Dresden, Germany, Max Planck Institute for Chemical Physics of Solids Dresden, Germany