Entropy transport in Bi$_{2}$Se$_{3}$

ORAL

Abstract

Bi$_2$Se$_3$ and Bi$_2$Te$_3$ are well known compounds in the thermoelectricity community as they present a high figure of merit [1]. Although the thermoelectric power of Bi$_2$Se$_3$ has been extensively studied at high temperature, little is known about its behaviour at the low temperature limit. In this presentation, we will report the results of our entropy measurement of Bi$_{2}$Se$_{3}$ at low temperature and high magnetic field for a bulk carrier concentration from 10$^{17}$cm$^3$ to 10$^{19}$cm$^3$. In all compounds we show significant quantum oscillations in the Seebeck and Nernst responses. Based on the bulk Fermi surface, we propose a simple description of the entropy transport measurement in Bi$_2$Se$_3$ (in the range of concentrations studied). Indeed, Bi$_2$Se$_3$ (non compensated system) appears as a complementary system of bismuth [2] and graphite [3] (compensated systems) to understand the entropy transport in the low carrier concentration limit. \\[4pt] [1] G.S. Nolas et al, Thermoelectrics Basic Principles and New Materials Developments, Springer.\\[0pt] [2] K.Behnia et al, PRL, 98, 166602 (2007)\\[0pt] [3] Z.Zhu et al, Nature Physics, 6, 26 (2009)

Authors

  • Beno\^it Fauqu\'e

    ESPCI, LPEM (UPMC-CNRS), ESPCI, 75005 Paris, France

  • Aurelie Collaudin

    LPEM (UPMC-CNRS), ESPCI, 75005 Paris, France

  • Kamran Behnia

    ESPCI, LPEM (UPMC-CNRS), ESPCI, 75005 Paris, France

  • Nick Butch

    Center for Nanophysics and Advanced Materials, Department of Physics, University of Maryland, College Park, Maryland 20742, USA

  • Johnpierre Palione

    University of Maryland, Center for Nanophysics and Advanced Materials, Department of Physics, University of Maryland-College Park, Center for Nanophysics and Advanced Materials, Dept. of Physics, University of Maryland, College Park, MD 20742, University of Maryland, College Park, Center for Nanophysics and Advanced Materials, Department of Physics, University of Maryland, College Park, Maryland 20742, USA, Center for Nanophysics and Advanced Materials, Physics Dept., University of Maryland, Center for Nanophysics \& Advanced Materials and Department of Physics, University of Maryland

  • Steffen Wiedmann

    High Field Magnet Laboratory, Institute for Molecules and Materials, Radboud University Nijmegen, 6525 ED Nijmegen, The Netherlands