Strong Electronic Correlations in YMn$_{2}$Ge$_{2}$

ORAL

Abstract

Exotic phases, like superconductivity, often emerge near electron delocalization transitions in strongly interacting systems. Magnetization, heat capacity and resistivity measurements were performed on single crystals of the antiferromagnetic metal YMn$_{2}$Ge$_{2}$, which is isostructural to the ThCr$_{2}$Si$_{2}$-type iron pnictides. Above the antiferromagnetic ordering temperature T$_{N}$=425 K, the magnetic susceptibility displays Curie-Weiss like behaviour with a fluctuating moment $\mu$ = 3.3 $\mu_{B}$/Mn atom, larger than the ordered moment of 2.2 $\mu_{B}$/Mn atom. Heat capacity measurements yield a Sommerfeld coefficient $\gamma$ = $\frac{C}{T}$ = 8.5 mJ/mol Mn K$^{2}$, nearly three times larger than $\gamma_{Ru}$ = 3.3 mJ/mol Mn K$^{2}$ for its non-magnetic isostructual analog YRu$_{2}$Ge$_{2}$, indicating strong electronic correlations in YMn$_{2}$Ge$_{2}$. The quasiparticle mass enhancement $\frac{m*}{m_{Ru}}$ = $\frac{\gamma}{\gamma_{Ru}}$ = 2.6 is similar to the value observed in the 122-type iron pinctides. Fermi-liquid behaviour of the resistivity $\rho = \rho_{0} + A T^{2}$ is observed over a very broad range of temperatures between 0.5 K and 300 K, with the resistivity at low temperature $\rho$(0.5 K) = 8 $\mu\Omega$ cm indicating high sample quality

Authors

  • Daniel McNally

    Department of Physics and Astronomy, Stony Brook University, Stony Brook, NY 11794, USA

  • J.W. Simonson

    Physics and Astronomy Dept., Stony Brook University, Department of Physics and Astronomy, Stony Brook University, Stony Brook, NY 11794, USA, Department of Physics and Astronomy, Stony Brook University

  • G. Smith

    Physics and Astronomy Dept., Stony Brook University, Department of Physics and Astronomy, Stony Brook University, Stony Brook, NY 11794, USA, Department of Physics and Astronomy, Stony Brook University

  • M.C. Aronson

    Physics and Astronomy Dept., Stony Brook University, Stony Brook University and Brookhaven National Laboratory, Department of Physics and Astronomy, Stony Brook University, Stony Brook, NY 11794, USA, Department of Physics and Astronomy, Stony Brook University