High-resolution RIXS measurement at O K-edge on the edge-shared chain cuprates, Ca$_{2+x}$Y$_{2-x}$Cu$_{5}$O$_{10}$
ORAL
Abstract
Quasi one dimensional copper oxides have been model systems in the field of correlated electron physics, because of rich phenomena exhibited in a relatively simple geometry. Its magnetic ground states, fluctuations, and excitations have been investigated extensively by theorists and experimentalists. Among the known quasi 1-D spin-chain compounds, Ca$_{2+x}$Y$_{2-x}$Cu$_{5}$O$_{10}$ is the only compound that can be hole-doped in a wide doping range, providing a unique opportunity to study the dynamics of hole in the quasi-1D environment. Here, we report ultrahigh resolution resonant inelastic soft x-ray scattering experiment at the O K-edge. With an energy resolution of $\sim $50 meV, we resolved rich charge excitations in the sub-eV range that has not been observed in the previous RIXS measurement on the same materials. In particular, we have resolved clear multi-phonon excitations near the elastic peak, suggesting a strong electron-phonon coupling in this quasi-1D system. Doping dependence of these excitations will also be demonstrated.
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Authors
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W.S. Lee
SLAC/ RSXS collaboration, SIMES, SLAC National Accelerator Lab.
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J. Lee
Stanford University
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M. Yi
Stanford University
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K. Zhou
Swiss Light Source, PSI
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Steven Johnston
IFW Dresden, IFW Dresden.
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T. Schmitt
Swiss Light Source, PSI
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Jeroen van den Brink
IFW, Dresden, IFW Dresden, IFW Dresden, Germany
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T.P. Devereaux
Stanford/SLAC, Stanford University and SLAC, SIMES, SLAC National Accelerator Laboratory, SIMES, SLAC National Accelerator Lab., Stanford University
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K. Kudo
Tohoku University
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Y. Koike
Tohoku University
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Luc Patthey
Swiss Light Source, PSI, PSI
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Z.-X. Shen
Stanford University, Geballe Laboratory for Advanced Materials, Departments of Physics and Applied Physics, Stanford University, CA 94305, SIMES, SLAC National Accelerator Lab.