High-resolution RIXS measurement at O K-edge on the edge-shared chain cuprates, Ca$_{2+x}$Y$_{2-x}$Cu$_{5}$O$_{10}$

ORAL

Abstract

Quasi one dimensional copper oxides have been model systems in the field of correlated electron physics, because of rich phenomena exhibited in a relatively simple geometry. Its magnetic ground states, fluctuations, and excitations have been investigated extensively by theorists and experimentalists. Among the known quasi 1-D spin-chain compounds, Ca$_{2+x}$Y$_{2-x}$Cu$_{5}$O$_{10}$ is the only compound that can be hole-doped in a wide doping range, providing a unique opportunity to study the dynamics of hole in the quasi-1D environment. Here, we report ultrahigh resolution resonant inelastic soft x-ray scattering experiment at the O K-edge. With an energy resolution of $\sim $50 meV, we resolved rich charge excitations in the sub-eV range that has not been observed in the previous RIXS measurement on the same materials. In particular, we have resolved clear multi-phonon excitations near the elastic peak, suggesting a strong electron-phonon coupling in this quasi-1D system. Doping dependence of these excitations will also be demonstrated.

Authors

  • W.S. Lee

    SLAC/ RSXS collaboration, SIMES, SLAC National Accelerator Lab.

  • J. Lee

    Stanford University

  • M. Yi

    Stanford University

  • K. Zhou

    Swiss Light Source, PSI

  • Steven Johnston

    IFW Dresden, IFW Dresden.

  • T. Schmitt

    Swiss Light Source, PSI

  • Jeroen van den Brink

    IFW, Dresden, IFW Dresden, IFW Dresden, Germany

  • T.P. Devereaux

    Stanford/SLAC, Stanford University and SLAC, SIMES, SLAC National Accelerator Laboratory, SIMES, SLAC National Accelerator Lab., Stanford University

  • K. Kudo

    Tohoku University

  • Y. Koike

    Tohoku University

  • Luc Patthey

    Swiss Light Source, PSI, PSI

  • Z.-X. Shen

    Stanford University, Geballe Laboratory for Advanced Materials, Departments of Physics and Applied Physics, Stanford University, CA 94305, SIMES, SLAC National Accelerator Lab.