Spin Dynamics and Electron-Phonon Coupling in Cuprates Measured by Resonant Inelastic X-Ray Scattering

ORAL

Abstract

We show how Resonant Inelastic X-ray Scattering (RIXS) is able to measure not only the dispersion of collective electronic and magnetic excitations in High Tc cuprates [1], but also their coupling to the lattice. At the Cu L$_3$ edge we observe the collective magnetic modes of La$_2$CuO$_4$ (LCO) and underdoped La$_{2-x}$Sr$_x$CuO$_4$ (LSCO) [2,3]. In LCO the single magnon dispersion measured by RIXS coincides with the one determined by inelastic neutron scattering. For LSCO the spin dynamics shows a branch dispersing up to $\sim$400 meV coexisting with a branch at lower energy [3]. Only the latter has been observed with neutrons so far and is considered a key signature of doped cuprates. The presence of the high-energy branch indicates that LSCO is in a dynamic inhomogeneous spin state. RIXS also provides direct, momentum-resolved information on the coupling between electrons and phonons. With it, we determine the e-p coupling strength of the Cu-O breathing mode in La$_2$CuO$_4$ and show that this coupling is strong enough to bring the material close to the polaron self-trapping regime when it is lightly doped with holes. [1] L. Ament {\it et. al.}, PRL 103, 117003 (2009). [2] L. Braicovich {\it et. al.}, PRL 102, 167401 (2009) [3] L. Braicovich {\it et. al.}, ArXiv:0911.0621 (2009).

Authors

  • Jeroen van den Brink

    Leibniz Institute IFW Dresden, Germany

  • Luuk Ament

    Leiden University, The Netherlands

  • Lucio Braicovich

    Politecnico di Milano, Italy

  • Giacomo Ghiringhelli

    Politecnico di Milano, Politecnico di Milano, Italy